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Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride
Chen, Jiayi1; Ge, Yao1,2; Guo, Yuanyuan1; Chen, Jinzhu1,3
2018
发表期刊JOURNAL OF ENERGY CHEMISTRY
ISSN2095-4956
卷号27期号:1页码:283-289
通讯作者Chen, Jinzhu(chenjz@jnu.edu.cn)
摘要Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural (HMF) to 2,5-dihydroxymethyl-tetrahydrofuran (DHMTHF) with 96% selectivity and a complete HMF conversion is obtained over palladium catalyst supported on mesoporous graphitic carbon nitride (Pd/mpg-C3N4) under pressured hydrogen atmosphere in aqueous media. The excellent catalytic performance of Pd/ mpg-C3N4 is attributed to hydrogen bonding-related competitive interactions between reactant HMF and "intermediate" 2,5-dihydroxymethylfuran (DHMF) with the support mpg-C3N4, which leads to a deep hydrogenation of DHMF to DHMTHF. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
关键词Biomass Carbon nitride 5-Hydroxymethylfurfural Hydrogenation
DOI10.1016/j.jechem.2017.04.017
关键词[WOS]RENEWABLE RESOURCES ; ALLOY CATALYST ; CYCLIC ETHERS ; DERIVATIVES ; CONVERSION ; HYDROGENOLYSIS ; PHENOL ; DEHYDRATION ; MORPHOLOGY ; REDUCTION
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[21472189] ; Science and Technology Planning Project of Guangzhou City, China[201707010238] ; Jinan Double Hundred Talents Plan
WOS研究方向Chemistry ; Energy & Fuels ; Engineering
项目资助者National Natural Science Foundation of China ; Science and Technology Planning Project of Guangzhou City, China ; Jinan Double Hundred Talents Plan
WOS类目Chemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000425889900029
出版者ELSEVIER SCIENCE BV
引用统计
被引频次:28[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/21374
专题中国科学院广州能源研究所
通讯作者Chen, Jinzhu
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Xinjiang Univ, Coll Chem & Chem Engn, Urumqi 830046, Xinjiang, Peoples R China
3.Jinan Univ, Coll Chem & Mat Sci, Guangzhou 510632, Guangdong, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Chen, Jiayi,Ge, Yao,Guo, Yuanyuan,et al. Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride[J]. JOURNAL OF ENERGY CHEMISTRY,2018,27(1):283-289.
APA Chen, Jiayi,Ge, Yao,Guo, Yuanyuan,&Chen, Jinzhu.(2018).Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride.JOURNAL OF ENERGY CHEMISTRY,27(1),283-289.
MLA Chen, Jiayi,et al."Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride".JOURNAL OF ENERGY CHEMISTRY 27.1(2018):283-289.
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