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Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride
Chen, Jiayi1; Ge, Yao1,2; Guo, Yuanyuan1; Chen, Jinzhu1,3
2018
Source PublicationJOURNAL OF ENERGY CHEMISTRY
ISSN2095-4956
Volume27Issue:1Pages:283-289
Corresponding AuthorChen, Jinzhu(chenjz@jnu.edu.cn)
AbstractSelective hydrogenation of biomass-derived 5-hydroxymethylfurfural (HMF) to 2,5-dihydroxymethyl-tetrahydrofuran (DHMTHF) with 96% selectivity and a complete HMF conversion is obtained over palladium catalyst supported on mesoporous graphitic carbon nitride (Pd/mpg-C3N4) under pressured hydrogen atmosphere in aqueous media. The excellent catalytic performance of Pd/ mpg-C3N4 is attributed to hydrogen bonding-related competitive interactions between reactant HMF and "intermediate" 2,5-dihydroxymethylfuran (DHMF) with the support mpg-C3N4, which leads to a deep hydrogenation of DHMF to DHMTHF. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
KeywordBiomass Carbon nitride 5-Hydroxymethylfurfural Hydrogenation
DOI10.1016/j.jechem.2017.04.017
WOS KeywordRENEWABLE RESOURCES ; ALLOY CATALYST ; CYCLIC ETHERS ; DERIVATIVES ; CONVERSION ; HYDROGENOLYSIS ; PHENOL ; DEHYDRATION ; MORPHOLOGY ; REDUCTION
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[21472189] ; Science and Technology Planning Project of Guangzhou City, China[201707010238] ; Jinan Double Hundred Talents Plan
WOS Research AreaChemistry ; Energy & Fuels ; Engineering
Funding OrganizationNational Natural Science Foundation of China ; Science and Technology Planning Project of Guangzhou City, China ; Jinan Double Hundred Talents Plan
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
WOS IDWOS:000425889900029
PublisherELSEVIER SCIENCE BV
Citation statistics
Cited Times:12[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/21374
Collection中国科学院广州能源研究所
Corresponding AuthorChen, Jinzhu
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Xinjiang Univ, Coll Chem & Chem Engn, Urumqi 830046, Xinjiang, Peoples R China
3.Jinan Univ, Coll Chem & Mat Sci, Guangzhou 510632, Guangdong, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Chen, Jiayi,Ge, Yao,Guo, Yuanyuan,et al. Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride[J]. JOURNAL OF ENERGY CHEMISTRY,2018,27(1):283-289.
APA Chen, Jiayi,Ge, Yao,Guo, Yuanyuan,&Chen, Jinzhu.(2018).Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride.JOURNAL OF ENERGY CHEMISTRY,27(1),283-289.
MLA Chen, Jiayi,et al."Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride".JOURNAL OF ENERGY CHEMISTRY 27.1(2018):283-289.
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