Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride | |
Chen, Jiayi1; Ge, Yao1,2; Guo, Yuanyuan1; Chen, Jinzhu1,3
| |
| 2018 | |
| Source Publication | JOURNAL OF ENERGY CHEMISTRY
 |
| ISSN | 2095-4956 |
| Volume | 27Issue:1Pages:283-289 |
| Corresponding Author | Chen, Jinzhu(chenjz@jnu.edu.cn) |
| Abstract | Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural (HMF) to 2,5-dihydroxymethyl-tetrahydrofuran (DHMTHF) with 96% selectivity and a complete HMF conversion is obtained over palladium catalyst supported on mesoporous graphitic carbon nitride (Pd/mpg-C3N4) under pressured hydrogen atmosphere in aqueous media. The excellent catalytic performance of Pd/ mpg-C3N4 is attributed to hydrogen bonding-related competitive interactions between reactant HMF and "intermediate" 2,5-dihydroxymethylfuran (DHMF) with the support mpg-C3N4, which leads to a deep hydrogenation of DHMF to DHMTHF. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved. |
| Keyword | Biomass Carbon nitride 5-Hydroxymethylfurfural Hydrogenation |
| DOI | 10.1016/j.jechem.2017.04.017 |
| WOS Keyword | RENEWABLE RESOURCES ; ALLOY CATALYST ; CYCLIC ETHERS ; DERIVATIVES ; CONVERSION ; HYDROGENOLYSIS ; PHENOL ; DEHYDRATION ; MORPHOLOGY ; REDUCTION |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | National Natural Science Foundation of China[21472189] ; Science and Technology Planning Project of Guangzhou City, China[201707010238] ; Jinan Double Hundred Talents Plan |
| WOS Research Area | Chemistry ; Energy & Fuels ; Engineering |
| Funding Organization | National Natural Science Foundation of China ; Science and Technology Planning Project of Guangzhou City, China ; Jinan Double Hundred Talents Plan |
| WOS Subject | Chemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical |
| WOS ID | WOS:000425889900029 |
| Publisher | ELSEVIER SCIENCE BV |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/21374 |
| Collection | 中国科学院广州能源研究所 |
| Corresponding Author | Chen, Jinzhu |
| Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 2.Xinjiang Univ, Coll Chem & Chem Engn, Urumqi 830046, Xinjiang, Peoples R China 3.Jinan Univ, Coll Chem & Mat Sci, Guangzhou 510632, Guangdong, Peoples R China |
| First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
| Recommended Citation GB/T 7714 | Chen, Jiayi,Ge, Yao,Guo, Yuanyuan,et al. Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride[J]. JOURNAL OF ENERGY CHEMISTRY,2018,27(1):283-289. |
| APA | Chen, Jiayi,Ge, Yao,Guo, Yuanyuan,&Chen, Jinzhu.(2018).Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride.JOURNAL OF ENERGY CHEMISTRY,27(1),283-289. |
| MLA | Chen, Jiayi,et al."Selective hydrogenation of biomass-derived 5-hydroxymethylfurfural using palladium catalyst supported on mesoporous graphitic carbon nitride".JOURNAL OF ENERGY CHEMISTRY 27.1(2018):283-289. |
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