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Promoted activity of porous silica coated Ni/Ceo(2)-Zro(2) catalyst for steam reforming of acetic acid
Zhao, Xiaoyong1,2,3; Xue, Yaping1; Yan, Changfeng1,2,3; Huang, Ting1; Lu, Zhuoxin1; Wang, Zhida1; Zhang, Liang1; Guo, Changqing1,2
2017-08-24
Source PublicationINTERNATIONAL JOURNAL OF HYDROGEN ENERGY
Volume42Issue:34Pages:21677-21685
AbstractPorous silica coated Ni/CeO2-ZrO2 catalysts were synthesized for steam reforming of acetic acid. The silica coated Ni/CeO2-ZrO2 catalyst showed a significantly enhanced activity (95% acetic acid conversion) than the Ni/CeO2-ZrO2 catalysts (62% acetic acid conversion) at a low temperature (550 degrees C). Interaction between Ni/CeO2-ZrO2 and silica layer was proved to be a crucial role on enhancing of catalytic activities. Further characterization (XPS, H-2-TPR) indicates this interaction facilitates the steam reforming reaction and raises the selectivity of CO by modifying the surface Ni electronic structure. In addition, the coated catalyst also exhibited a good stability and no obvious deactivation was detected at 550 degrees C and 600 degrees C within 30 h. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
SubtypeArticle
KeywordBiomass Bio-oil Acetic Acid Steam Reforming Hydrogen Production
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1016/j.ijhydene.2017.07.086
WOS Subject ExtendedChemistry ; Electrochemistry ; Energy & Fuels
WOS KeywordOIL MODEL COMPOUNDS ; GAS SHIFT REACTION ; HYDROGEN-PRODUCTION ; BIO-OIL ; NICKEL-CATALYSTS ; NI CATALYST ; BED REACTOR ; THERMODYNAMIC ANALYSIS ; NI/CE-ZRO2 CATALYST ; METAL CATALYSTS
Indexed BySCI
Language英语
Funding OrganizationNatural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong Province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2016201604030010)
WOS SubjectChemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS IDWOS:000411545300011
Citation statistics
Cited Times:20[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/16302
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Zhao, Xiaoyong,Xue, Yaping,Yan, Changfeng,et al. Promoted activity of porous silica coated Ni/Ceo(2)-Zro(2) catalyst for steam reforming of acetic acid[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2017,42(34):21677-21685.
APA Zhao, Xiaoyong.,Xue, Yaping.,Yan, Changfeng.,Huang, Ting.,Lu, Zhuoxin.,...&Guo, Changqing.(2017).Promoted activity of porous silica coated Ni/Ceo(2)-Zro(2) catalyst for steam reforming of acetic acid.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,42(34),21677-21685.
MLA Zhao, Xiaoyong,et al."Promoted activity of porous silica coated Ni/Ceo(2)-Zro(2) catalyst for steam reforming of acetic acid".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 42.34(2017):21677-21685.
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