Effect of Hydrate Saturation on the Methane Hydrate Dissociation by Depressurization in Sediments in a Cubic Hydrate Simulator

doi:10.1021/ie5042885

GIEC OpenIR > 中国科学院广州能源研究所

	Effect of Hydrate Saturation on the Methane Hydrate Dissociation by Depressurization in Sediments in a Cubic Hydrate Simulator
	Zhang, Yu; Li, Xiao-Sen1 ; Chen, Zhao-Yang ; Wang, Yi ; Ruan, Xu-Ke
	2015-03-18
发表期刊	INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷号	54 期号:10 页码:2627-2637
摘要	This study presents the three-dimensional (3D) cubic hydrate simulator (CHS) to analyze the methane dissociation phenomena from hydrate-bearing sediment with different hydrate saturation. The experiments by depressurization have been carried out at the environmental temperature of 281.15 K, the dissociation pressure of 5.0 MPa, and in the hydrate saturation range of 17.0-43.2%. The hydrate dissociation process consists of two periods: the depressurizing period and the steady-pressure period: In the depressurizing period, the hydrate dissociation occurs in the whole reactor. The cumulative gas production is similar, and the gas production rate is affected by the depressurization rate and the water production in this period. The cumulative water production increases With the decrease of the hydrate saturation in the whole depressurization process. In the steady-pressure period, the cumulative gas production increases with the increase of the hydrate saturation. The average gas production rate first increases with the increase of the hydrate saturation and then decreases at hydrate saturation of 43.2%. The water production during the steady-pressure period only occurs in the experiments with the high hydrate saturation. The temperatures in different regions in the reactor change with similar degrees in the depressurizing period and have the similar lowest values for different experiments. In the steady-pressure period, the temperatures increase gradually from the inner-wall region to the center region. On the basis of the calculation of the energy balance, it was found that the ratio of the sensible heat of the reservoir to the latent heat of the hydrate dissociation decreases with the increases of the hydrate saturation and the dissociation pressure.
文章类型	Article
WOS标题词	Science & Technology ; Technology
DOI	10.1021/ie5042885
研究领域[WOS]	Engineering
关键词[WOS]	GAS HYDRATE ; PRODUCTION BEHAVIOR ; POROUS SEDIMENTS ; SEA ; PRODUCTIVITY ; INJECTION ; SCHEME ; MEDIA
收录类别	SCI
语种	英语
WOS类目	Engineering, Chemical
WOS记录号	WOS:000351420600006
引用统计	被引频次：29[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/9093
专题	中国科学院广州能源研究所
作者单位	1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China 2.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
推荐引用方式 GB/T 7714	Zhang, Yu,Li, Xiao-Sen,Chen, Zhao-Yang,et al. Effect of Hydrate Saturation on the Methane Hydrate Dissociation by Depressurization in Sediments in a Cubic Hydrate Simulator[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2015,54(10):2627-2637.
APA	Zhang, Yu,Li, Xiao-Sen,Chen, Zhao-Yang,Wang, Yi,&Ruan, Xu-Ke.(2015).Effect of Hydrate Saturation on the Methane Hydrate Dissociation by Depressurization in Sediments in a Cubic Hydrate Simulator.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,54(10),2627-2637.
MLA	Zhang, Yu,et al."Effect of Hydrate Saturation on the Methane Hydrate Dissociation by Depressurization in Sediments in a Cubic Hydrate Simulator".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 54.10(2015):2627-2637.