Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point

doi:10.1002/ep.13953

GIEC OpenIR

	Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point
	Zhang, Xuemin 1,2,3; Yang, Huijie 1,2; Li, Jinping 1,2; Zhang, Mengjun 1,2; Wang, Yingmei 1,2,4; Yao, Ze 1,2
	2022-07-29
发表期刊	ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY
ISSN	1944-7442
页码	11
通讯作者	Zhang, Xuemin(zxm2010lut@163.com)
摘要	The formation process of gas hydrate is a stochastic phenomenon considered to be significant for its application in the areas such as hydrate-based technology and natural gas hydrate exploitation. The formation behaviors of CO2 hydrate were studied in porous media below the freezing point. In addition, the formation experiments were conducted in the high-pressure vessel under different temperature and pressure conditions. The formation process of CO2 hydrate showed different formation behaviors in the porous media under different experimental conditions. The results showed that the formation rate was higher in earlier stage and the largest formation rate attained 7.18 x 10(-4) mol h(-1). The influence of initial pressure on the formation rate was indistinctive in porous media below the freezing point. Particle size of the porous media played an important role in affecting the formation characteristic of CO2 hydrate below the freezing point. The results indicated that, the smaller the particle size of porous media was, the larger the formation rate and the conversion rate of CO2 hydrate. The maximum conversion rate was attained 90.61%. The results also indicated that CO2 hydrate had a good gas storage capacity in porous media below the freezing point. The gas storage capacity was close to 160 L/L in frozen quartz sand with the particle size of 250 mu m in the experiments. The relative results will provide some insight for sequestration and storage process of CO2 gas in the form of hydrates into sediments.
关键词	carbon dioxide storage CO2 hydrate formation behavior freezing point porous media
DOI	10.1002/ep.13953
关键词[WOS]	GAS-HYDRATE ; CLATHRATE HYDRATE ; METHANE ; CAPTURE ; STORAGE ; DISSOCIATION ; ICE ; IMPACT ; GROWTH ; CRYSTALLIZATION
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51906093] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[Y907ke1001] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[E029kf1501] ; Lanzhou University of Technology
WOS研究方向	Science & Technology - Other Topics ; Engineering ; Environmental Sciences & Ecology
项目资助者	National Natural Science Foundation of China ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences ; Lanzhou University of Technology
WOS类目	Green & Sustainable Science & Technology ; Engineering, Environmental ; Engineering, Chemical ; Environmental Sciences
WOS记录号	WOS:000832619700001
出版者	WILEY
引用统计
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/36990
专题	中国科学院广州能源研究所
通讯作者	Zhang, Xuemin
作者单位	1.Lanzhou Univ Technol, Western China Res Ctr Energy & Environm, Lanzhou 730050, Peoples R China 2.Key Lab Complementary Energy Syst Biomass & Solar, Lanzhou, Gansu, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou, Guangdong, Peoples R China 4.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Frozen Soil Engn, Lanzhou, Peoples R China
第一作者单位	中国科学院广州能源研究所
推荐引用方式 GB/T 7714	Zhang, Xuemin,Yang, Huijie,Li, Jinping,et al. Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point[J]. ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,2022:11.
APA	Zhang, Xuemin,Yang, Huijie,Li, Jinping,Zhang, Mengjun,Wang, Yingmei,&Yao, Ze.(2022).Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point.ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,11.
MLA	Zhang, Xuemin,et al."Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point".ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY (2022):11.