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Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point
Zhang, Xuemin1,2,3; Yang, Huijie1,2; Li, Jinping1,2; Zhang, Mengjun1,2; Wang, Yingmei1,2,4; Yao, Ze1,2
2022-07-29
Source PublicationENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY
ISSN1944-7442
Pages11
Corresponding AuthorZhang, Xuemin(zxm2010lut@163.com)
AbstractThe formation process of gas hydrate is a stochastic phenomenon considered to be significant for its application in the areas such as hydrate-based technology and natural gas hydrate exploitation. The formation behaviors of CO2 hydrate were studied in porous media below the freezing point. In addition, the formation experiments were conducted in the high-pressure vessel under different temperature and pressure conditions. The formation process of CO2 hydrate showed different formation behaviors in the porous media under different experimental conditions. The results showed that the formation rate was higher in earlier stage and the largest formation rate attained 7.18 x 10(-4) mol h(-1). The influence of initial pressure on the formation rate was indistinctive in porous media below the freezing point. Particle size of the porous media played an important role in affecting the formation characteristic of CO2 hydrate below the freezing point. The results indicated that, the smaller the particle size of porous media was, the larger the formation rate and the conversion rate of CO2 hydrate. The maximum conversion rate was attained 90.61%. The results also indicated that CO2 hydrate had a good gas storage capacity in porous media below the freezing point. The gas storage capacity was close to 160 L/L in frozen quartz sand with the particle size of 250 mu m in the experiments. The relative results will provide some insight for sequestration and storage process of CO2 gas in the form of hydrates into sediments.
Keywordcarbon dioxide storage CO2 hydrate formation behavior freezing point porous media
DOI10.1002/ep.13953
WOS KeywordGAS-HYDRATE ; CLATHRATE HYDRATE ; METHANE ; CAPTURE ; STORAGE ; DISSOCIATION ; ICE ; IMPACT ; GROWTH ; CRYSTALLIZATION
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51906093] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[Y907ke1001] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[E029kf1501] ; Lanzhou University of Technology
WOS Research AreaScience & Technology - Other Topics ; Engineering ; Environmental Sciences & Ecology
Funding OrganizationNational Natural Science Foundation of China ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences ; Lanzhou University of Technology
WOS SubjectGreen & Sustainable Science & Technology ; Engineering, Environmental ; Engineering, Chemical ; Environmental Sciences
WOS IDWOS:000832619700001
PublisherWILEY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/36990
Collection中国科学院广州能源研究所
Corresponding AuthorZhang, Xuemin
Affiliation1.Lanzhou Univ Technol, Western China Res Ctr Energy & Environm, Lanzhou 730050, Peoples R China
2.Key Lab Complementary Energy Syst Biomass & Solar, Lanzhou, Gansu, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou, Guangdong, Peoples R China
4.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Frozen Soil Engn, Lanzhou, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Zhang, Xuemin,Yang, Huijie,Li, Jinping,et al. Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point[J]. ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,2022:11.
APA Zhang, Xuemin,Yang, Huijie,Li, Jinping,Zhang, Mengjun,Wang, Yingmei,&Yao, Ze.(2022).Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point.ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,11.
MLA Zhang, Xuemin,et al."Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point".ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY (2022):11.
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