Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point | |
Zhang, Xuemin1,2,3; Yang, Huijie1,2; Li, Jinping1,2; Zhang, Mengjun1,2; Wang, Yingmei1,2,4; Yao, Ze1,2 | |
2022-07-29 | |
Source Publication | ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY
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ISSN | 1944-7442 |
Pages | 11 |
Corresponding Author | Zhang, Xuemin(zxm2010lut@163.com) |
Abstract | The formation process of gas hydrate is a stochastic phenomenon considered to be significant for its application in the areas such as hydrate-based technology and natural gas hydrate exploitation. The formation behaviors of CO2 hydrate were studied in porous media below the freezing point. In addition, the formation experiments were conducted in the high-pressure vessel under different temperature and pressure conditions. The formation process of CO2 hydrate showed different formation behaviors in the porous media under different experimental conditions. The results showed that the formation rate was higher in earlier stage and the largest formation rate attained 7.18 x 10(-4) mol h(-1). The influence of initial pressure on the formation rate was indistinctive in porous media below the freezing point. Particle size of the porous media played an important role in affecting the formation characteristic of CO2 hydrate below the freezing point. The results indicated that, the smaller the particle size of porous media was, the larger the formation rate and the conversion rate of CO2 hydrate. The maximum conversion rate was attained 90.61%. The results also indicated that CO2 hydrate had a good gas storage capacity in porous media below the freezing point. The gas storage capacity was close to 160 L/L in frozen quartz sand with the particle size of 250 mu m in the experiments. The relative results will provide some insight for sequestration and storage process of CO2 gas in the form of hydrates into sediments. |
Keyword | carbon dioxide storage CO2 hydrate formation behavior freezing point porous media |
DOI | 10.1002/ep.13953 |
WOS Keyword | GAS-HYDRATE ; CLATHRATE HYDRATE ; METHANE ; CAPTURE ; STORAGE ; DISSOCIATION ; ICE ; IMPACT ; GROWTH ; CRYSTALLIZATION |
Indexed By | SCI |
Language | 英语 |
Funding Project | National Natural Science Foundation of China[51906093] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[Y907ke1001] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[E029kf1501] ; Lanzhou University of Technology |
WOS Research Area | Science & Technology - Other Topics ; Engineering ; Environmental Sciences & Ecology |
Funding Organization | National Natural Science Foundation of China ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences ; Lanzhou University of Technology |
WOS Subject | Green & Sustainable Science & Technology ; Engineering, Environmental ; Engineering, Chemical ; Environmental Sciences |
WOS ID | WOS:000832619700001 |
Publisher | WILEY |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.giec.ac.cn/handle/344007/36990 |
Collection | 中国科学院广州能源研究所 |
Corresponding Author | Zhang, Xuemin |
Affiliation | 1.Lanzhou Univ Technol, Western China Res Ctr Energy & Environm, Lanzhou 730050, Peoples R China 2.Key Lab Complementary Energy Syst Biomass & Solar, Lanzhou, Gansu, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou, Guangdong, Peoples R China 4.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Frozen Soil Engn, Lanzhou, Peoples R China |
First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
Recommended Citation GB/T 7714 | Zhang, Xuemin,Yang, Huijie,Li, Jinping,et al. Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point[J]. ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,2022:11. |
APA | Zhang, Xuemin,Yang, Huijie,Li, Jinping,Zhang, Mengjun,Wang, Yingmei,&Yao, Ze.(2022).Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point.ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY,11. |
MLA | Zhang, Xuemin,et al."Investigation of the formation behaviors of CO2 hydrate in porous media below the freezing point".ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY (2022):11. |
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