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Construction of hierarchical Fe2O3@MnO2 core/shell nanocube supported C3N4 for dual Z-scheme photocatalytic water splitting | |
Wang, Nan; Wu, Liangpeng![]() ![]() ![]() | |
2020-09-15 | |
Source Publication | SOLAR ENERGY MATERIALS AND SOLAR CELLS
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ISSN | 0927-0248 |
Volume | 215Pages:8 |
Corresponding Author | Li, Xinjun(lixj@ms.giec.ac.cn) |
Abstract | A dual Z-scheme fe(2)O(3)@MnO2 core/shell nanocube supported C3N4 ternary composite is rationally designed and successfully fabricated as a photocatalyst for water splitting. The as-prepared Fe2O3@MnO2/C3N4 ternary composite exhibits an enhanced visible light-induced absorbance capacity and superior photocatalytic activity for direct water splitting than that of pure g-C3N4. The photocatalytic efficiency is investigated by varying amounts of Fe2O3@MnO2/shell nanocubes in the ternary composite (10%wt, 20%wt and 30%wt). When the mass fraction of Fe2O3@MnO2 is determined to be 20%, the hydrogen evolution rate would achieve the maximum with a value of 124 mu mol*h(-1). The improved photocatalytic performance of Fe2O3@MnO2 ternary composite can be mainly attributed to improved visible light absorption range and construction of an effective dual Z-scheme interfacial heterojunction with a rapid separation and transfer of electron-hole pairs. |
Keyword | Z-scheme heterostructure Fe2O3@MnO2 nanocube Core-shell, Photocatalytic water splitting |
DOI | 10.1016/j.solmat.2020.110624 |
WOS Keyword | COMPOSITE ; HETEROSTRUCTURE ; DEGRADATION ; PERFORMANCE ; NANOSHEETS ; NANOSCALE |
Indexed By | SCI |
Language | 英语 |
Funding Project | Science and Technology Program of Guangzhou, China[201803030019] ; Analysis and Testing Center of Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences |
WOS Research Area | Energy & Fuels ; Materials Science ; Physics |
Funding Organization | Science and Technology Program of Guangzhou, China ; Analysis and Testing Center of Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences |
WOS Subject | Energy & Fuels ; Materials Science, Multidisciplinary ; Physics, Applied |
WOS ID | WOS:000574947000012 |
Publisher | ELSEVIER |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.giec.ac.cn/handle/344007/32093 |
Collection | 中国科学院广州能源研究所 |
Corresponding Author | Li, Xinjun |
Affiliation | Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China |
First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
Recommended Citation GB/T 7714 | Wang, Nan,Wu, Liangpeng,Li, Juan,et al. Construction of hierarchical Fe2O3@MnO2 core/shell nanocube supported C3N4 for dual Z-scheme photocatalytic water splitting[J]. SOLAR ENERGY MATERIALS AND SOLAR CELLS,2020,215:8. |
APA | Wang, Nan,Wu, Liangpeng,Li, Juan,Mo, Jiamei,Peng, Quanming,&Li, Xinjun.(2020).Construction of hierarchical Fe2O3@MnO2 core/shell nanocube supported C3N4 for dual Z-scheme photocatalytic water splitting.SOLAR ENERGY MATERIALS AND SOLAR CELLS,215,8. |
MLA | Wang, Nan,et al."Construction of hierarchical Fe2O3@MnO2 core/shell nanocube supported C3N4 for dual Z-scheme photocatalytic water splitting".SOLAR ENERGY MATERIALS AND SOLAR CELLS 215(2020):8. |
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