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Methane hydrate formation and dissociation behaviors in montmorillonite
Yan, Kefeng; Li, Xiaosen1; Chen, Zhaoyang; Zhang, Yu; Xu, Chungang; Xia, Zhiming
2019-05-01
Source PublicationCHINESE JOURNAL OF CHEMICAL ENGINEERING
ISSN1004-9541
Volume27Issue:5Pages:1212-1218
Corresponding AuthorLi, Xiaosen(lixs@ms.giec.ac.cn)
AbstractThe methane hydrate formation and the methane hydrate dissociation behaviors in montmorillonite arc experimentally studied. Through the analyses of the microstructure characteristic, the study obtains the porous characteristic of montmorillonite. It is indicated that methane hydrate in montmorillonite forms the structure I (sI) crystal. Meanwhile, molecular dynamics simulation is carried out to study the processes of the methane hydrate formation and the methane hydrate dissociation in montmorillonite. The microstructure and microscopic properties are analyzed. The methane hydrate formation and methane hydrate dissociation mechanisms in the montmorillonite nanopore and on the montmorillonite surface arc expounded. Combining the experimental and simulating analyses, the results indicate the methane hydrate formation and methane hydrate dissociation processes have little influence upon the crystal structure of porous media from either micro- or macro-analysis. It is beneficial to the fundamental researches on the exploitation and security control technologies of natural gas hydrate in deep-sea sediments. (C) 2018 The Chemical Industry and Engineering Society of China, and Chemical Industry Press Co., Ltd. All rights reserved.
KeywordMethane hydrate Porous media Formation/dissociation behavior Molecular dynamics simulation
DOI10.1016/j.cjche.2018.11.025
WOS KeywordMOLECULAR-DYNAMICS SIMULATIONS ; WATER ; NUCLEATION ; CAPTURE ; CO2 ; SEPARATION ; SURFACES ; MODELS
Indexed BySCI
Language英语
Funding ProjectGuangzhou Branch of the Supercomputing Center of Chinese Academy of Sciences ; Guangzhou Branch of the Supercomputer Center of the Computer Network Information Center, Chinese Academy of Sciences
WOS Research AreaEngineering
Funding OrganizationGuangzhou Branch of the Supercomputing Center of Chinese Academy of Sciences ; Guangzhou Branch of the Supercomputer Center of the Computer Network Information Center, Chinese Academy of Sciences
WOS SubjectEngineering, Chemical
WOS IDWOS:000472199000029
PublisherCHEMICAL INDUSTRY PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/25247
Corresponding AuthorLi, Xiaosen
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
Recommended Citation
GB/T 7714
Yan, Kefeng,Li, Xiaosen,Chen, Zhaoyang,et al. Methane hydrate formation and dissociation behaviors in montmorillonite[J]. CHINESE JOURNAL OF CHEMICAL ENGINEERING,2019,27(5):1212-1218.
APA Yan, Kefeng,Li, Xiaosen,Chen, Zhaoyang,Zhang, Yu,Xu, Chungang,&Xia, Zhiming.(2019).Methane hydrate formation and dissociation behaviors in montmorillonite.CHINESE JOURNAL OF CHEMICAL ENGINEERING,27(5),1212-1218.
MLA Yan, Kefeng,et al."Methane hydrate formation and dissociation behaviors in montmorillonite".CHINESE JOURNAL OF CHEMICAL ENGINEERING 27.5(2019):1212-1218.
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