Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method

doi:10.1039/c9ra02090j

GIEC OpenIR

	Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method
	Mei, Qun 1,2; Wei, Xiangqian 1; Sun, Weitao 1; Zhang, Xinghua2 ; Li, Wenzhi 1; Ma, Longlong2
	2019
发表期刊	RSC ADVANCES
ISSN	2046-2069
卷号	9 期号:23 页码:12846-12853
通讯作者	Li, Wenzhi(liwenzhi@ustc.edu.cn) ; Ma, Longlong(mall@ms.giec.ac.cn)
摘要	Conversion of cellulose to 5-hydroxymethylfurfural (HMF) is an important means of biomass utilization. However, simulation of hydrolysis of cellulose and species transport in multiphase systems is still missing. In this paper, a multiphase lattice Boltzmann method of the Shan-Chen model has been applied for simulating the complex chemical reactions and interphase mass transfer in a liquid membrane catalytic reactor. For the sake of simplification, a single particle liquid membrane catalytic model is developed to simulate the hydrolysis of cellulose into HMF and its side reactions, which include the adsorption of cellulose particles on the liquid membrane, the complex chemical reactions inside the liquid membrane and the interphase transfer of HMF. This simulation presents the results of hydrolysis of cellulose and the HMF transport process. Additionally, the results show that the thinner liquid membrane thickness is beneficial for increasing the yield of HMF.
DOI	10.1039/c9ra02090j
关键词[WOS]	BIOMASS FAST PYROLYSIS ; MASS-TRANSFER ; SIMULATION ; DEHYDRATION ; CONVERSION ; FRUCTOSE ; ZEOLITE ; FLOW
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51576198] ; National Natural Science Foundation of China[51536009] ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21060102]
WOS研究方向	Chemistry
项目资助者	National Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences
WOS类目	Chemistry, Multidisciplinary
WOS记录号	WOS:000468636000008
出版者	ROYAL SOC CHEMISTRY
引用统计	被引频次：4[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/24979
专题	中国科学院广州能源研究所
通讯作者	Li, Wenzhi; Ma, Longlong
作者单位	1.Univ Sci & Technol China, Dept Thermal Sci & Energy Engn, Lab Basic Res Biomass Convers & Utilizat, Hefei 230026, Anhui, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
第一作者单位	中国科学院广州能源研究所
推荐引用方式 GB/T 7714	Mei, Qun,Wei, Xiangqian,Sun, Weitao,et al. Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method[J]. RSC ADVANCES,2019,9(23):12846-12853.
APA	Mei, Qun,Wei, Xiangqian,Sun, Weitao,Zhang, Xinghua,Li, Wenzhi,&Ma, Longlong.(2019).Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method.RSC ADVANCES,9(23),12846-12853.
MLA	Mei, Qun,et al."Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method".RSC ADVANCES 9.23(2019):12846-12853.