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Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method
Mei, Qun1,2; Wei, Xiangqian1; Sun, Weitao1; Zhang, Xinghua2; Li, Wenzhi1; Ma, Longlong2
2019
Source PublicationRSC ADVANCES
ISSN2046-2069
Volume9Issue:23Pages:12846-12853
Corresponding AuthorLi, Wenzhi(liwenzhi@ustc.edu.cn) ; Ma, Longlong(mall@ms.giec.ac.cn)
AbstractConversion of cellulose to 5-hydroxymethylfurfural (HMF) is an important means of biomass utilization. However, simulation of hydrolysis of cellulose and species transport in multiphase systems is still missing. In this paper, a multiphase lattice Boltzmann method of the Shan-Chen model has been applied for simulating the complex chemical reactions and interphase mass transfer in a liquid membrane catalytic reactor. For the sake of simplification, a single particle liquid membrane catalytic model is developed to simulate the hydrolysis of cellulose into HMF and its side reactions, which include the adsorption of cellulose particles on the liquid membrane, the complex chemical reactions inside the liquid membrane and the interphase transfer of HMF. This simulation presents the results of hydrolysis of cellulose and the HMF transport process. Additionally, the results show that the thinner liquid membrane thickness is beneficial for increasing the yield of HMF.
DOI10.1039/c9ra02090j
WOS KeywordBIOMASS FAST PYROLYSIS ; MASS-TRANSFER ; SIMULATION ; DEHYDRATION ; CONVERSION ; FRUCTOSE ; ZEOLITE ; FLOW
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51576198] ; National Natural Science Foundation of China[51536009] ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21060102]
WOS Research AreaChemistry
Funding OrganizationNational Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000468636000008
PublisherROYAL SOC CHEMISTRY
Citation statistics
Cited Times:5[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/24979
Collection中国科学院广州能源研究所
Corresponding AuthorLi, Wenzhi; Ma, Longlong
Affiliation1.Univ Sci & Technol China, Dept Thermal Sci & Energy Engn, Lab Basic Res Biomass Convers & Utilizat, Hefei 230026, Anhui, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Mei, Qun,Wei, Xiangqian,Sun, Weitao,et al. Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method[J]. RSC ADVANCES,2019,9(23):12846-12853.
APA Mei, Qun,Wei, Xiangqian,Sun, Weitao,Zhang, Xinghua,Li, Wenzhi,&Ma, Longlong.(2019).Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method.RSC ADVANCES,9(23),12846-12853.
MLA Mei, Qun,et al."Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method".RSC ADVANCES 9.23(2019):12846-12853.
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