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CO2气氛下生物质焦气化反应动力学模型研究:Ⅱ.指数前因子
Alternative TitleModeling study on the biomass char gasification kinetics under CO2 atmosphere:Ⅱ. Pre-exponential factor
汪小憨1,2; 宋谦石1,3; 曾小军1,2; 吴勇1,3
2017-05
Source Publication燃料化学学报
ISSN0253-2409
Volume45Issue:5Pages:529-536
Abstract基于简单碰撞理论,建立了生物质焦炭CO2气化反应速率的计算方法,找出了表征指数前因子大小的关键组合参数。在此基础上,对六种生物质及其脱灰焦炭的物理化学特性进行了检测分析,利用热重分析仪在800-1 000℃对各种生物质进行了CO2等温气化实验,将得到的指数前因子实验数据与模型分析结果进行对比。研究表明,指数前因子与构建的组合参数之间存在较好的相关性,建立的通用关系式可为气化反应规律的进一步阐明提供有益的参考。
Other AbstractBased on the simple collision theory(SCT),the calculation method of biomass char gasification rate was developed and the combined parameters to characterize the pre-exponential factor were found. Furthermore,some experimental tests for six acid-washed biomass chars,such as the isothermal gasification and so on,were performed under CO2 atmosphere,using a thermo-gravimetric analyzer(TGA) over the temperature ranges of 800-1 000 ℃,respectively. Through the comparison of experimental data and modeling results,it is found that a good agreement is made and the developed model equations can provide an effective guidance to clarify the general gasification law of biomass chars.
Keyword生物质焦炭 CO2气化 简单碰撞理论 指数前因子 模型研究 biomass char CO2 gasification simple collision theory pre-exponential factor modelling
Language中文
CSCD IDCSCD:5991650
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/16520
Collection中国科学院广州能源研究所
Corresponding Author汪小憨
Affiliation1.中国科学院广州能源研究所,广东广州510640;
2.中国科学院可再生能源重点实验室,广东广州510640;
3.中国科学院大学,北京100049
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
汪小憨,宋谦石,曾小军,等. CO2气氛下生物质焦气化反应动力学模型研究:Ⅱ.指数前因子[J]. 燃料化学学报,2017,45(5):529-536.
APA 汪小憨,宋谦石,曾小军,&吴勇.(2017).CO2气氛下生物质焦气化反应动力学模型研究:Ⅱ.指数前因子.燃料化学学报,45(5),529-536.
MLA 汪小憨,et al."CO2气氛下生物质焦气化反应动力学模型研究:Ⅱ.指数前因子".燃料化学学报 45.5(2017):529-536.
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