Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules

doi:10.1021/acsami.7b11940

GIEC OpenIR

	Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules
	Huang, Qizhang 1,3; Fang, Yueyun 1,3; Shi, Jifu1,2 ; Liang, Yanliang 4,5; Zhu, Yanqing1 ; Xu, Gang1,6
	2017-10-18
发表期刊	ACS APPLIED MATERIALS & INTERFACES
ISSN	1944-8244
卷号	9 期号:41 页码:36431-36437
摘要	Flower-like molybdenum disulfide (MoS2) with rich edge sites has been prepared by the hydrothermal method. The edge sites possess polarity due to the noncentrosymmetric Mo-S on exposed (100) facets and thus show a strong electrostatic attraction toward polar species. The flower-like MoS2 can be used as small-molecule carriers for the model drug, Rhodamine B (RhB). The results prove that flower-like MoS2 have fast adsorption kinetics and perform a switchable accumulation/release with response to the solvent polarity. An outstanding reusability can be found in flower-like MoS2 due to little cargo retention, and the recycle of adsorption can be repeated 100 times with above 88.5% of the adsorption capacity retained. The flower-like MoS2 with solvent polarity-triggered loading/release can be extended to controlled release and color switch of display.
文章类型	Article
关键词	Molybdenum Disulfide Polarity Reusability Adsorption Solvents
WOS标题词	Science & Technology ; Technology
DOI	10.1021/acsami.7b11940
研究领域[WOS]	Science & Technology - Other Topics ; Materials Science
关键词[WOS]	DRUG-RELEASE ; RHODAMINE-B ; MOS2 NANOSTRUCTURES ; HYDROGEN EVOLUTION ; AQUEOUS-SOLUTION ; METHYLENE-BLUE ; WATER ; ADSORPTION ; ADSORBENT ; REMOVAL
收录类别	SCI
语种	英语
项目资助者	National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017)
WOS类目	Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000413503700097
出版者	AMER CHEMICAL SOC
引用统计	被引频次：44[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/16503
专题	中国科学院广州能源研究所
通讯作者	Shi, Jifu; Liang, Yanliang; Xu, Gang
作者单位	1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China 2.Jinan Univ, Dept Phys, Siyuan Lab, Guangzhou 510632, Guangdong, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.Univ Houston, Dept Elect & Comp Engn, Houston, TX 77204 USA 5.Univ Houston, Mat Sci & Engn Program, Houston, TX 77204 USA 6.Tibet New Energy Res & Demonstrat Ctr, Lhasa 850000, Tibet, Peoples R China
第一作者单位	中国科学院广州能源研究所
推荐引用方式 GB/T 7714	Huang, Qizhang,Fang, Yueyun,Shi, Jifu,et al. Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules[J]. ACS APPLIED MATERIALS & INTERFACES,2017,9(41):36431-36437.
APA	Huang, Qizhang,Fang, Yueyun,Shi, Jifu,Liang, Yanliang,Zhu, Yanqing,&Xu, Gang.(2017).Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules.ACS APPLIED MATERIALS & INTERFACES,9(41),36431-36437.
MLA	Huang, Qizhang,et al."Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules".ACS APPLIED MATERIALS & INTERFACES 9.41(2017):36431-36437.