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Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules
Huang, Qizhang1,3; Fang, Yueyun1,3; Shi, Jifu1,2; Liang, Yanliang4,5; Zhu, Yanqing1; Xu, Gang1,6
2017-10-18
Source PublicationACS APPLIED MATERIALS & INTERFACES
ISSN1944-8244
Volume9Issue:41Pages:36431-36437
AbstractFlower-like molybdenum disulfide (MoS2) with rich edge sites has been prepared by the hydrothermal method. The edge sites possess polarity due to the noncentrosymmetric Mo-S on exposed (100) facets and thus show a strong electrostatic attraction toward polar species. The flower-like MoS2 can be used as small-molecule carriers for the model drug, Rhodamine B (RhB). The results prove that flower-like MoS2 have fast adsorption kinetics and perform a switchable accumulation/release with response to the solvent polarity. An outstanding reusability can be found in flower-like MoS2 due to little cargo retention, and the recycle of adsorption can be repeated 100 times with above 88.5% of the adsorption capacity retained. The flower-like MoS2 with solvent polarity-triggered loading/release can be extended to controlled release and color switch of display.
SubtypeArticle
KeywordMolybdenum Disulfide Polarity Reusability Adsorption Solvents
WOS HeadingsScience & Technology ; Technology
DOI10.1021/acsami.7b11940
WOS Subject ExtendedScience & Technology - Other Topics ; Materials Science
WOS KeywordDRUG-RELEASE ; RHODAMINE-B ; MOS2 NANOSTRUCTURES ; HYDROGEN EVOLUTION ; AQUEOUS-SOLUTION ; METHYLENE-BLUE ; WATER ; ADSORPTION ; ADSORBENT ; REMOVAL
Indexed BySCI
Language英语
Funding OrganizationNational Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; National Natural Science Foundation of China(21673243) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Guangdong-Hong Kong Joint Innovation Project of Guangdong Province, China(2014B050505015) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Special Support Program of Guangdong Province, China(2014TQ01N610) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Project of Science and Technology Service Network initiative, Chinese Academy of Sciences(KFJ-STS-QYZD-010) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017) ; Tibet Autonomous Region Major Special Projects(ZD20170017)
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000413503700097
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:9[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/16503
Collection中国科学院广州能源研究所
Corresponding AuthorShi, Jifu; Liang, Yanliang; Xu, Gang
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
2.Jinan Univ, Dept Phys, Siyuan Lab, Guangzhou 510632, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Univ Houston, Dept Elect & Comp Engn, Houston, TX 77204 USA
5.Univ Houston, Mat Sci & Engn Program, Houston, TX 77204 USA
6.Tibet New Energy Res & Demonstrat Ctr, Lhasa 850000, Tibet, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Huang, Qizhang,Fang, Yueyun,Shi, Jifu,et al. Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules[J]. ACS APPLIED MATERIALS & INTERFACES,2017,9(41):36431-36437.
APA Huang, Qizhang,Fang, Yueyun,Shi, Jifu,Liang, Yanliang,Zhu, Yanqing,&Xu, Gang.(2017).Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules.ACS APPLIED MATERIALS & INTERFACES,9(41),36431-36437.
MLA Huang, Qizhang,et al."Flower-Like Molybdenum Disulfide for Polarity-Triggered Accumulation/Release of Small Molecules".ACS APPLIED MATERIALS & INTERFACES 9.41(2017):36431-36437.
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