GIEC OpenIR
Knitting Aryl Network Polymers-Incorporated Ag Nanoparticles: A Mild and Efficient Catalyst for the Fixation of CO2 as Carboxylic Acid
Wu, Zhilian1,2,4; Liu, Qinggang2; Yang, Xiaofeng2; Ye, Xue2; Duan, Hongmin2; Zhang, Jian2; Zhao, Bo3; Huang, Yanqiang2
2017-11-01
发表期刊ACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN2168-0485
卷号5期号:11页码:9634-9639
摘要A simple and scalable method for synthesizing silver nanoparticles supported on the framework of mesoporous knitting aryl network polymers (KAPs) has been developed. With the benefits from its mesoporous texture and the stabilizing effect of phosphine compounds in the matrix, the silver precursor can be efficiently introduced into the KAPs framework, which results in a nanosize distribution of Ag (ca. 4.1 nm) supported on KAPs (Ag/KAPs-P) with narrow particle size distribution and homogeneous dispersion after simple reduction step. The as-obtained metal small sized Ag/KAPs-P catalyst is particularly active for the direct carboxylation of terminal alkynes with CO2 into carboxylic acid at low temperature and atmospheric pressure. Moreover, this Ag/KAPs-P catalyst also shows high stability under the reaction conditions, and it can be recycled at least five times without significant loss of activity, suggesting its great potential application in the heterogeneous conversion of CO2 into carboxylic acid.
文章类型Article
关键词Carbon Dioxide Porous Organic Polymers Heterogeneous Catalyst Alkynyl Carboxylic Acid
WOS标题词Science & Technology ; Physical Sciences ; Technology
资助者National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269) ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269) ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269) ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269)
DOI10.1021/acssuschemeng.7b02678
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]METAL-ORGANIC FRAMEWORKS ; CARBON-DIOXIDE ; CHEMOSELECTIVE HYDROGENATION ; TERMINAL ALKYNES ; AMBIENT-PRESSURE ; MICROPOROUS POLYMERS ; AROMATIC KETONES ; SELECTIVITY ; CONVERSION ; CAPTURE
收录类别SCI
语种英语
资助者National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269) ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269) ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269) ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Natural Science Foundation of China(21403218 ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; National Key R&D Program of China(2016YFB0600902) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; State Grid Cooperation of China(SGRI-DL-71-16-016) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Dalian Science Foundation(2016RJ04) ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; 21476226 ; 21476226 ; 21476226 ; 21476226 ; 21503125 ; 21503125 ; 21503125 ; 21503125 ; 21506204 ; 21506204 ; 21506204 ; 21506204 ; 21776269) ; 21776269) ; 21776269) ; 21776269)
WOS类目Chemistry, Multidisciplinary ; Engineering, Chemical
WOS记录号WOS:000414825900013
出版者AMER CHEMICAL SOC
引用统计
被引频次:2[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/16481
专题中国科学院广州能源研究所
通讯作者Yang, Xiaofeng; Huang, Yanqiang
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, 2 Nengyuan Rd,Wushan St, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, State Key Lab Catalysis, iChEM Collaborat Innovat Ctr Chem Energy Mat, Dalian Inst Chem Phys, 457 Zhongshan Rd, Dalian 116023, Peoples R China
3.Global Energy Interconnect Res Inst, State Key Lab Adv Power Transmiss Technol, Beijing 102211, Peoples R China
4.Univ Chinese Acad Sci, 19 A Yuquan Rd, Beijing 100049, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Wu, Zhilian,Liu, Qinggang,Yang, Xiaofeng,et al. Knitting Aryl Network Polymers-Incorporated Ag Nanoparticles: A Mild and Efficient Catalyst for the Fixation of CO2 as Carboxylic Acid[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2017,5(11):9634-9639.
APA Wu, Zhilian.,Liu, Qinggang.,Yang, Xiaofeng.,Ye, Xue.,Duan, Hongmin.,...&Huang, Yanqiang.(2017).Knitting Aryl Network Polymers-Incorporated Ag Nanoparticles: A Mild and Efficient Catalyst for the Fixation of CO2 as Carboxylic Acid.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,5(11),9634-9639.
MLA Wu, Zhilian,et al."Knitting Aryl Network Polymers-Incorporated Ag Nanoparticles: A Mild and Efficient Catalyst for the Fixation of CO2 as Carboxylic Acid".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 5.11(2017):9634-9639.
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