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Py-GC/MS study of lignin pyrolysis and effect of catalysts on product distribution
Si Zhan1,2,3; Wang Chenguang2; Bi Kang2,4; Zhang Xinghua2; Yu Chiling5; Dong Renjie1,3,6; Ma Longlong2; Pang Changle7
2017-09-01
发表期刊INTERNATIONAL JOURNAL OF AGRICULTURAL AND BIOLOGICAL ENGINEERING
ISSN1934-6344
卷号10期号:5页码:214-225
摘要Fast pyrolysis is one of the most promising methods to convert lignin into fuels and chemicals. In the present study, pyrolysis-gas chromatography/mass spectrometry (Py-GC/MS) was used to evaluate vapor phase product distribution of lignin fast pyrolysis. During the non-catalytic pyrolysis process, lignin was pyrolyzed at 400 degrees C, 500 degrees C and 600 degrees C respectively, finding that the highest yield of aromatic hydrocarbons was obtained at 600 degrees C. Catalytic pyrolysis experiments were also conducted to investigate the effects of catalyst pore structure and acidity on the product distributions. Five different catalysts (HZSM-5, MCM-41, TiO2, ZrO2 and Mg(Al) O) were applied to lignin catalytic pyrolysis, and the catalytic performance was estimated by analyzing the pyrolytic products. The catalysts were characterized by using X-ray diffraction ( XRD), BET, and NH3 (CO2) temperature programmed desorption. Based on these characterizations, discussion was carried out to explain the formation of the produc distributions. Among the five catalysts, HZSM-5 exhibited the best performance on the formation of aromatic hydrocarbons.
文章类型Article
关键词Lignin Py-gc/ms Fast Pyrolysis Catalytic Upgrading Pore Structure Acid-base Property
WOS标题词Science & Technology ; Life Sciences & Biomedicine
资助者National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering ; National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering ; National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering ; National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering
DOI10.25165/j.ijabe.20171005.2852
研究领域[WOS]Agriculture
关键词[WOS]FLUIDIZED-BED REACTOR ; BIOMASS PYROLYSIS ; SHAPE SELECTIVITY ; KRAFT LIGNIN ; FUELS ; CHEMICALS ; ZEOLITE ; HYDROCARBONS ; CONVERSION ; ACIDITY
收录类别SCI
语种英语
资助者National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering ; National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering ; National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering ; National Natural Science Foundation of China(51536009) ; National Natural Science Foundation of China(51536009) ; NSFC (Natural Science Foundation of China) project(51476175) ; NSFC (Natural Science Foundation of China) project(51476175) ; National Basic Research Program of China(2013CB228105) ; National Basic Research Program of China(2013CB228105) ; Chinese Academy of Sciences "one hundred talented plan" ; Chinese Academy of Sciences "one hundred talented plan" ; Beijing Municipal Key Discipline of Biomass Engineering ; Beijing Municipal Key Discipline of Biomass Engineering
WOS类目Agricultural Engineering
WOS记录号WOS:000412990100021
出版者CHINESE ACAD AGRICULTURAL ENGINEERING
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/16388
专题生物质化工品制备实验室
生物质能研究中心
作者单位1.China Agr Univ, Coll Engn, Bioenergy & Environm Sci & Technol Lab, Beijing 100083, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
3.Minist Agr, Key Lab Clean Prod & Utilizat Renewable Energy, Beijing 100083, Peoples R China
4.Zhengzhou Univ, Sch Chem Engn & Energy, Zhengzhou 450001, Henan, Peoples R China
5.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
6.Minist Sci & Technol, Natl Ctr Int Res BioEnergy Sci & Technol, Beijing 100083, Peoples R China
7.China Agr Univ, Dept Vehicle Engn, Coll Engn, Beijing 100083, Peoples R China
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Si Zhan,Wang Chenguang,Bi Kang,et al. Py-GC/MS study of lignin pyrolysis and effect of catalysts on product distribution[J]. INTERNATIONAL JOURNAL OF AGRICULTURAL AND BIOLOGICAL ENGINEERING,2017,10(5):214-225.
APA Si Zhan.,Wang Chenguang.,Bi Kang.,Zhang Xinghua.,Yu Chiling.,...&Pang Changle.(2017).Py-GC/MS study of lignin pyrolysis and effect of catalysts on product distribution.INTERNATIONAL JOURNAL OF AGRICULTURAL AND BIOLOGICAL ENGINEERING,10(5),214-225.
MLA Si Zhan,et al."Py-GC/MS study of lignin pyrolysis and effect of catalysts on product distribution".INTERNATIONAL JOURNAL OF AGRICULTURAL AND BIOLOGICAL ENGINEERING 10.5(2017):214-225.
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