Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
The transformation pathways of nitrogen in sewage sludge during hydrothermal treatment | |
Zhuang, Xiuzheng1,2,3,4; Huang, Yanqin1,2,3; Song, Yanpei1,2,3,4; Zhan, Hao1,2,3,4; Yin, Xiuli1,2,3; Wu, Chuangzhi1,2,3 | |
2017-12-01 | |
Source Publication | BIORESOURCE TECHNOLOGY |
ISSN | 0960-8524 |
Volume | 245Pages:463-470 |
Abstract | Hydrothermal treatment (HT) has been proved as a significant pretreatment in decreasing emissions of NOX pollutants from thermochemical utilization of sewage sludge (SS) derived solid fuel. This study aims to investigate the denitrification of HT and the redistribution of nitrogen (N) in different products so as to speculate the comprehensive pathway of N transformation during hydrothermal process. Results found that only 20% of N remained in hydrochar, whereas the rest of N (nearly 80%) was transformed into other phase. A majority of amino-N in SS was enriched in liquid phase in the form of Org-N at first, then further decomposed to NH4+-N. The remaining amino-N converted to pyrrole-N, pyridine-N and quaternary-N as temperature progresses. Meanwhile, amine-N derived from protein-N formed heterocyclic-N in oil phase via Diels-Alder reaction. NH3, the major nitrogenous gas, was dissolved in liquid as NH4+-N immediately after producing, but increased with prolonged reaction time. |
Subtype | Article |
Keyword | Transformation Pathways Hydrothermal Treatment Denitrification Sewage Sludge |
WOS Headings | Science & Technology ; Life Sciences & Biomedicine ; Technology |
DOI | 10.1016/j.biortech.2017.08.195 |
WOS Subject Extended | Agriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels |
WOS Keyword | INDUSTRIAL BIOMASS WASTES ; FT-IR SPECTROSCOPY ; NO EMISSION ; MUNICIPAL SLUDGE ; MODEL COMPOUNDS ; LIQUEFACTION ; PYROLYSIS ; COMBUSTION ; CONVERSION ; RECOVERY |
Indexed By | SCI |
Language | 英语 |
Funding Organization | National Natural Science Foundation of China(51676195 ; National Natural Science Foundation of China(51676195 ; 51661145022) ; 51661145022) ; National Natural Science Foundation of China(51676195 ; National Natural Science Foundation of China(51676195 ; 51661145022) ; 51661145022) |
WOS Subject | Agricultural Engineering ; Biotechnology & Applied Microbiology ; Energy & Fuels |
WOS ID | WOS:000412443500059 |
Publisher | ELSEVIER SCI LTD |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.giec.ac.cn/handle/344007/16383 |
Collection | 生物质热化学转化实验室 |
Corresponding Author | Yin, Xiuli |
Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Beijing, Peoples R China 2.CAS Key Lab Renewable Energy, Beijing, Peoples R China 3.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou, Guangdong, Peoples R China 4.Univ Chinese Acad Sci, Beijing 10049, Peoples R China |
First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
Recommended Citation GB/T 7714 | Zhuang, Xiuzheng,Huang, Yanqin,Song, Yanpei,et al. The transformation pathways of nitrogen in sewage sludge during hydrothermal treatment[J]. BIORESOURCE TECHNOLOGY,2017,245:463-470. |
APA | Zhuang, Xiuzheng,Huang, Yanqin,Song, Yanpei,Zhan, Hao,Yin, Xiuli,&Wu, Chuangzhi.(2017).The transformation pathways of nitrogen in sewage sludge during hydrothermal treatment.BIORESOURCE TECHNOLOGY,245,463-470. |
MLA | Zhuang, Xiuzheng,et al."The transformation pathways of nitrogen in sewage sludge during hydrothermal treatment".BIORESOURCE TECHNOLOGY 245(2017):463-470. |
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