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Encapsulating Ni/CeO2-ZrO2 with SiO2 layer to improve it catalytic activity for steam reforming of toluene
Zhao, Xiaoyong1,2,3; Xue, Yaping1; Lu, Zhuoxin1; Huang, Ying1; Guo, Changqing1; Yan, Changfeng1,2,3
2017-11-01
发表期刊CATALYSIS COMMUNICATIONS
卷号101页码:138-141
摘要Ni/CeO2-ZrO2 was encapsulated by SiO2 layer with expectation to obtain a high active catalyst for steam reforming of toluene. The coating structure was validated by X-ray diffraction experiments and electron microscope analysis. XPS data suggests the formation of a new Ni-O-Si configuration in core-shell catalysts. The presence of Ni-O-Si configuration shift electron from Ni to silica and thereby facilitates the intrinsic properties of catalysts. Compared to Ni/CeO2-ZrO2, turnover rate of Ni increased substantially in core-shell structures, Ni/CeO2-ZrO2@SiO2 with shell-to-core mass ratio as 1.0 showed about 5.5 times higher than the Ni/CeO2-ZrO2 catalyst.
文章类型Article
关键词Biomass Tar Toluene Steam Reforming Core-shell Catalyst
WOS标题词Science & Technology ; Physical Sciences
资助者Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong Province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2016201604030010) ; Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong Province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2016201604030010)
DOI10.1016/j.catcom.2017.08.013
研究领域[WOS]Chemistry
关键词[WOS]GAS SHIFT CATALYSIS ; NI-BASED CATALYSTS ; BIOMASS TAR ; MODEL-COMPOUND ; HYDROGEN-PRODUCTION ; NICKEL-CATALYSTS ; PRODUCER GAS ; GASIFICATION ; CONVERSION ; SUPPORT
收录类别SCI
语种英语
资助者Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong Province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2016201604030010) ; Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong Province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2016201604030010)
WOS类目Chemistry, Physical
WOS记录号WOS:000411552400031
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/16305
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
推荐引用方式
GB/T 7714
Zhao, Xiaoyong,Xue, Yaping,Lu, Zhuoxin,et al. Encapsulating Ni/CeO2-ZrO2 with SiO2 layer to improve it catalytic activity for steam reforming of toluene[J]. CATALYSIS COMMUNICATIONS,2017,101:138-141.
APA Zhao, Xiaoyong,Xue, Yaping,Lu, Zhuoxin,Huang, Ying,Guo, Changqing,&Yan, Changfeng.(2017).Encapsulating Ni/CeO2-ZrO2 with SiO2 layer to improve it catalytic activity for steam reforming of toluene.CATALYSIS COMMUNICATIONS,101,138-141.
MLA Zhao, Xiaoyong,et al."Encapsulating Ni/CeO2-ZrO2 with SiO2 layer to improve it catalytic activity for steam reforming of toluene".CATALYSIS COMMUNICATIONS 101(2017):138-141.
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