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Influence of Carbon Dioxide on the Thermal Degradation Process of Representative Components of Combustible Solid Wastes Using Thermogravimetric-Mass Spectrometry
Gu, J.1,2; Wang, Y. Z.1,2; Yuan, H. R.1,2; Huhe, T. L.1,2; Chen, Y.1,2,3
2017-08-01
发表期刊ENERGY & FUELS
卷号31期号:8页码:8317-8325
摘要The thermal mass loss, gaseous-phase reactions, and reaction-kinetics, of five representative components of combustible solid wastes (CSWs), i.e., rice straw (RS), eucalyptus wood, blank printing paper (BPP), high-density polyethylene, and polyvinyl chloride (PVC), under argon (Ar) and carbon dioxide (CO2) atmospheres-were studied by thermogravimetric mass spectrometry toobserve the effect of CO, on the thermal degradation process The CO2 atmosphere had a bigger influence than the Ar atmosphere on the thermal mass loss of CSW; CO, affected the main gaseous product distribution, which was attributed to the-complex gas reforming reaction that occurred in the, gaseous-phase, arid:abundant CO2 promoted the formation of CO and CH4:-Whentheteinperatute was over 650 degrees C, the CO2 reduction reaction occurred in the solidphase and the residue of RS and BPP was mainly silicon, calcium, and potassium oxidizers. The best fitting mechanism of the first main mass loss stage of CSW in an Ar atmosphere was mainly the nucleation and growth model. The best fitting mechanism of the second main mass loss of biomass-based combustible solid wastes under a CO2 atmosphere was the diffuion model, anclthat- of plastic combustible solid wastes was, the reaction order model. Furthermore, dehydrochlorination of PVC occurred at 200-384 C,, wherein chlorine atoms were released iii different compound forms under Ar and CO2 atmospheres: Therefore, the emissions from the heat treatment of CSW under a CO2 atmosphere presented an improved environinental profile tompaied to those released from pyrolysis under an Ar atmosphere.
文章类型Article
WOS标题词Science & Technology ; Technology
资助者National Natural Science Foundation of China(51406207 ; Biomass Energy and Materials Key Laboratory Open Fund of Jiangsu Province(JSBEM201609) ; Chinese Academy of Sciences Scientific Research and Equipment Development Project(YZ201516) ; Guangdong Science-Technology Project(2015A020209115 ; 51606202) ; 2015B090904009) ; National Natural Science Foundation of China(51406207 ; Biomass Energy and Materials Key Laboratory Open Fund of Jiangsu Province(JSBEM201609) ; Chinese Academy of Sciences Scientific Research and Equipment Development Project(YZ201516) ; Guangdong Science-Technology Project(2015A020209115 ; 51606202) ; 2015B090904009)
DOI10.1021/acs.energyfuels.7b01226
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]LIGNOCELLULOSIC BIOMASS ; ENERGY RECOVERY ; RICE STRAW ; PYROLYSIS ; GASIFICATION ; CO2 ; DECOMPOSITION ; KINETICS ; LIGNIN ; MODEL
收录类别SCI
语种英语
资助者National Natural Science Foundation of China(51406207 ; Biomass Energy and Materials Key Laboratory Open Fund of Jiangsu Province(JSBEM201609) ; Chinese Academy of Sciences Scientific Research and Equipment Development Project(YZ201516) ; Guangdong Science-Technology Project(2015A020209115 ; 51606202) ; 2015B090904009) ; National Natural Science Foundation of China(51406207 ; Biomass Energy and Materials Key Laboratory Open Fund of Jiangsu Province(JSBEM201609) ; Chinese Academy of Sciences Scientific Research and Equipment Development Project(YZ201516) ; Guangdong Science-Technology Project(2015A020209115 ; 51606202) ; 2015B090904009)
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000408178100062
引用统计
被引频次:2[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/16294
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Div Acad, Guangzhou 510070, Guangdong, Peoples R China
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Gu, J.,Wang, Y. Z.,Yuan, H. R.,et al. Influence of Carbon Dioxide on the Thermal Degradation Process of Representative Components of Combustible Solid Wastes Using Thermogravimetric-Mass Spectrometry[J]. ENERGY & FUELS,2017,31(8):8317-8325.
APA Gu, J.,Wang, Y. Z.,Yuan, H. R.,Huhe, T. L.,&Chen, Y..(2017).Influence of Carbon Dioxide on the Thermal Degradation Process of Representative Components of Combustible Solid Wastes Using Thermogravimetric-Mass Spectrometry.ENERGY & FUELS,31(8),8317-8325.
MLA Gu, J.,et al."Influence of Carbon Dioxide on the Thermal Degradation Process of Representative Components of Combustible Solid Wastes Using Thermogravimetric-Mass Spectrometry".ENERGY & FUELS 31.8(2017):8317-8325.
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