Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| Sorbent assisted catalyst of Ni-CaO-La2O3 for sorption enhanced steam reforming of bio-oil with acetic acid as the model compound | |
Zhao, Xiao-yong1,2; Xue, Ya-ping1,2; Yan, Chang-feng1,2 ; Wang, Zhi-da1; Guo, Chang-qing1; Huang, Shi-lin1
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| 2017-09-01 | |
| Source Publication | CHEMICAL ENGINEERING AND PROCESSING
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| Volume | 119Pages:106-112 |
| Abstract | Sorption enhanced steam reforming of acetic acid over sorbent assisted catalyst of Ni-CaO-La2O3 were investigated for high-purity H-2 production. Ni-CaO-La2O3 with 8, 16 and 20 wt% Ni were developed by sol-gel combustion synthesis and were characterized by TG, TPR, BET, SEM, XRD and XPS. The catalytic activities and stability of the catalysts were tested in a fixed reactor. H-2 yield and H-2 concentration through Ni-CaO-La2O3 with 20 wt% Ni reaches 86.02% and 92.24% during pre-breakthrough period, respectively, which is attributed to sufficient Ni active sites on the surface and good Ni dispersion. Catalytic activities of Ni-CaO-La2O3 with 20 wt% Ni maintain stable during sorption-enhanced steam reforming reaction, but CO2 sorption capacity slightly decreases due to blockage of pores and size increase of CaO particles within nine sorption/desorption cycles. |
| Subtype | Article |
| Keyword | Sorbent Assisted Catalyst Ni-cao-la2o3 Acetic Acid Bio-oil Hydrogen Production Sorption Enhanced Steam Reforming |
| WOS Headings | Science & Technology ; Technology |
| DOI | 10.1016/j.cep.2017.05.012 |
| WOS Subject Extended | Energy & Fuels ; Engineering |
| WOS Keyword | HYDROGEN-PRODUCTION ; CO2 CAPTURE ; METHANE ; PERFORMANCE ; BIOMASS |
| Indexed By | SCI |
| Language | 英语 |
| WOS Subject | Energy & Fuels ; Engineering, Chemical |
| WOS ID | WOS:000406731000012 |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/16280 |
| Collection | 中国科学院广州能源研究所 |
| Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100039, Peoples R China |
| First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
| Recommended Citation GB/T 7714 | Zhao, Xiao-yong,Xue, Ya-ping,Yan, Chang-feng,et al. Sorbent assisted catalyst of Ni-CaO-La2O3 for sorption enhanced steam reforming of bio-oil with acetic acid as the model compound[J]. CHEMICAL ENGINEERING AND PROCESSING,2017,119:106-112. |
| APA | Zhao, Xiao-yong,Xue, Ya-ping,Yan, Chang-feng,Wang, Zhi-da,Guo, Chang-qing,&Huang, Shi-lin.(2017).Sorbent assisted catalyst of Ni-CaO-La2O3 for sorption enhanced steam reforming of bio-oil with acetic acid as the model compound.CHEMICAL ENGINEERING AND PROCESSING,119,106-112. |
| MLA | Zhao, Xiao-yong,et al."Sorbent assisted catalyst of Ni-CaO-La2O3 for sorption enhanced steam reforming of bio-oil with acetic acid as the model compound".CHEMICAL ENGINEERING AND PROCESSING 119(2017):106-112. |
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