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Alfalfa Leaf-Derived Porous Heteroatom-Doped Carbon Materials as Efficient Cathodic Catalysts in Microbial Fuel Cells
Deng, Lifang1,3,5; Yuan, Yong2; Zhang, Yuyuan4; Wang, Yazhuo3,5; Chen, Yong3,5; Yuan, Haoran3,4,5; Chen, Ying1
2017-11-01
发表期刊ACS SUSTAINABLE CHEMISTRY & ENGINEERING
卷号5期号:11页码:9766-9773
摘要Heteroatom-doped lamellar-structured carbon with a high surface area synthesized from alfalfa leaves is utilized as a cathode catalyst in this study to improve the power output of microbial fuel cells (MFCs). Different chemical activation agents are used to treat alfalfa leaf-derived carbon (ALC). It is found that chemical activation agents substantially affect the catalytic activities of the alfalfa leaf-derived carbon materials in the power output of MFCs and the oxygen reduction reaction (ORR). ALC materials activated by KOH (ALC-K) exhibit the best electrochemical activity compared with those of materials activated by FeCl3 (ALC-Fe) or ZnCl2 (ALC-Zn). A high limiting current density and excellent long-term stability can be seen with ALC-K as the cathode catalyst, which gives superior results to those of Pt/C. Moreover, a maximum power density of approximately 1328.9 mW/m(2) is obtained from an MFC equipped with an ALC-K cathode, offering performance characteristics comparable to those of a Pt/C cathode as well. This work demonstrates a new method for the production of inexpensive natural resources that exhibit high performance in MFCs.
文章类型Article
关键词Alfalfa Leaf-derived Carbon Oxygen Reduction Reaction Chemical Activation Microbial Fuel Cell
WOS标题词Science & Technology ; Physical Sciences ; Technology
资助者National Natural Science Foundation of China(51406207) ; Guangdong Natural Science Funds for Distinguished Young Scholars(2014A030306033) ; National science and technology support(2015BAL04B02) ; Guangzhou university-industry collaborative innovation major projects(2016201604030077) ; Cooperation Project of Industry-University-Research in Guangdong Province(2015B090904009) ; Youth Innovation Promotion Association CAS(2014320) ; National Natural Science Foundation of China(51406207) ; Guangdong Natural Science Funds for Distinguished Young Scholars(2014A030306033) ; National science and technology support(2015BAL04B02) ; Guangzhou university-industry collaborative innovation major projects(2016201604030077) ; Cooperation Project of Industry-University-Research in Guangdong Province(2015B090904009) ; Youth Innovation Promotion Association CAS(2014320)
DOI10.1021/acssuschemeng.7b01585
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]OXYGEN REDUCTION REACTION ; METAL-FREE ELECTROCATALYSTS ; ACTIVATED CARBON ; AIR-CATHODE ; CHEMICAL-COMPOSITION ; NEUTRAL MEDIA ; WASTE-WATER ; NITROGEN ; GRAPHENE ; IRON
收录类别SCI
语种英语
资助者National Natural Science Foundation of China(51406207) ; Guangdong Natural Science Funds for Distinguished Young Scholars(2014A030306033) ; National science and technology support(2015BAL04B02) ; Guangzhou university-industry collaborative innovation major projects(2016201604030077) ; Cooperation Project of Industry-University-Research in Guangdong Province(2015B090904009) ; Youth Innovation Promotion Association CAS(2014320) ; National Natural Science Foundation of China(51406207) ; Guangdong Natural Science Funds for Distinguished Young Scholars(2014A030306033) ; National science and technology support(2015BAL04B02) ; Guangzhou university-industry collaborative innovation major projects(2016201604030077) ; Cooperation Project of Industry-University-Research in Guangdong Province(2015B090904009) ; Youth Innovation Promotion Association CAS(2014320)
WOS类目Chemistry, Multidisciplinary ; Engineering, Chemical
WOS记录号WOS:000414825900030
引用统计
被引频次:2[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/15864
专题中国科学院广州能源研究所
作者单位1.Guangdong Univ Technol, Sch Mat & Energy, Guangzhou Higher Educ Mega Ctr, 100 Waihuan Xi Rd, Guangzhou 510006, Guangdong, Peoples R China
2.Guangdong Univ Technol, Sch Environm Sci & Engn, Guangzhou Higher Educ Mega Ctr, 100 Waihuan Xi Rd, Guangzhou 510006, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, 2 Nengyuan Rd, Guangzhou 510640, Guangdong, Peoples R China
4.Foshan Univ, Coll Mat Sci & Energy Engn, 18 Jiangwan Yi Rd, Foshan 528000, Peoples R China
5.Guangdong Prov Key Lab New & Renewable Energy Res, 2 Nengyuan Rd, Guangzhou 510640, Guangdong, Peoples R China
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Deng, Lifang,Yuan, Yong,Zhang, Yuyuan,et al. Alfalfa Leaf-Derived Porous Heteroatom-Doped Carbon Materials as Efficient Cathodic Catalysts in Microbial Fuel Cells[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2017,5(11):9766-9773.
APA Deng, Lifang.,Yuan, Yong.,Zhang, Yuyuan.,Wang, Yazhuo.,Chen, Yong.,...&Chen, Ying.(2017).Alfalfa Leaf-Derived Porous Heteroatom-Doped Carbon Materials as Efficient Cathodic Catalysts in Microbial Fuel Cells.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,5(11),9766-9773.
MLA Deng, Lifang,et al."Alfalfa Leaf-Derived Porous Heteroatom-Doped Carbon Materials as Efficient Cathodic Catalysts in Microbial Fuel Cells".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 5.11(2017):9766-9773.
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