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GLUCOSE-DERIVED CARBONACEOUS SOLID ACID CATALYST FOR CELLOOLIGOSACCHARIDES HYDROLYSIS IN AN AQUEOUS REACTION SYSTEM
Liu, Wan-Yu1; Qi, Wei2; Liu, Shu-Na2; Wang, Qiong2; Zhou, Jin-Song1; Yuan, Zhen-Hong2; Zhuang, Xin-Shu2
2017-05-01
发表期刊CELLULOSE CHEMISTRY AND TECHNOLOGY
卷号51期号:5-6页码:417-423
摘要An amorphous carbon based catalyst was prepared by carbonation and sulfonation of several typical biomass materials, including glucose, microcrystalline cellulose, sugarcane bagasse, eucalyptus, switchgrass and microalgae. Preliminary experimental results on cellobiose hydrolysis indicated that the catalyst prepared from glucose exhibited the highest catalytic activity. Thus, methods, including SEM, XRD, FT-IR, NH3-TPD and elemental analysis, were employed to characterize the catalyst before and after sulfonation. Compared with other conventional solid acid catalysts, the catalyst bearing -SO3H, -COOH, and -OH groups exhibited remarkable activity in the hydrolysis of beta-1,4-glycosidic bonds and no other by-reactions were detected in further hydrolysis experiments. After the hydrolysis reaction, the solid acid catalyst could be readily separated from the saccharide solution for reuse without any significant loss of activity.
文章类型Article
关键词Carbonaceous Solid Acid Hydrolysis Cellooligosaccharides
WOS标题词Science & Technology ; Technology
资助者National Natural Science Foundation(21376241 ; 51506207 ; 51561145015 ; 51206173) ; National Natural Science Foundation(21376241 ; 51506207 ; 51561145015 ; 51206173)
研究领域[WOS]Materials Science
关键词[WOS]IONIC LIQUID ; AMORPHOUS-CARBON ; CELLULOSE ; PRETREATMENT ; BAGASSE ; WATER
收录类别SCI
语种英语
资助者National Natural Science Foundation(21376241 ; 51506207 ; 51561145015 ; 51206173) ; National Natural Science Foundation(21376241 ; 51506207 ; 51561145015 ; 51206173)
WOS类目Materials Science, Paper & Wood
WOS记录号WOS:000413719200004
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/15863
专题中国科学院广州能源研究所
作者单位1.Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Zhejiang, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
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GB/T 7714
Liu, Wan-Yu,Qi, Wei,Liu, Shu-Na,et al. GLUCOSE-DERIVED CARBONACEOUS SOLID ACID CATALYST FOR CELLOOLIGOSACCHARIDES HYDROLYSIS IN AN AQUEOUS REACTION SYSTEM[J]. CELLULOSE CHEMISTRY AND TECHNOLOGY,2017,51(5-6):417-423.
APA Liu, Wan-Yu.,Qi, Wei.,Liu, Shu-Na.,Wang, Qiong.,Zhou, Jin-Song.,...&Zhuang, Xin-Shu.(2017).GLUCOSE-DERIVED CARBONACEOUS SOLID ACID CATALYST FOR CELLOOLIGOSACCHARIDES HYDROLYSIS IN AN AQUEOUS REACTION SYSTEM.CELLULOSE CHEMISTRY AND TECHNOLOGY,51(5-6),417-423.
MLA Liu, Wan-Yu,et al."GLUCOSE-DERIVED CARBONACEOUS SOLID ACID CATALYST FOR CELLOOLIGOSACCHARIDES HYDROLYSIS IN AN AQUEOUS REACTION SYSTEM".CELLULOSE CHEMISTRY AND TECHNOLOGY 51.5-6(2017):417-423.
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