Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| Mild Hydrogenation of Lignin Depolymerization Products Over Ni/SiO2 Catalyst | |
Shu, Riyang1,2,3,4; Xu, Ying1,2,3 ; Chen, Pengru1,2,3,4; Ma, Longlong1,2,3; Zhang, Qi1,2,3; Zhou, Lie1,2,3; Wang, Chenguang1,2,3
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| 2017-07-01 | |
| Source Publication | ENERGY & FUELS
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| Volume | 31Issue:7Pages:7208-7213 |
| Abstract | Many efficient methods have been proposed to realize lignin depolymerization, while effective usage of lignin depolymerization products at mild conditions is still a big challenge. Conversion of them to stable products in thermal and chemical properties is a necessary step. Herein, a mild hydrogenation process of lignin depolymerization products over Ni/SiO2 catalyst was proposed. Model compound of 2,3-dihydrobenzofuran exhibited a good reaction result. Nearly 100% conversion was obtained at 130 degrees C, and the selectivity of 2-ethylcyclohexanol product reached 94.6%. The lignin depolymerization products also had a good hydrogenation result, in which not only the hydrogenation of unsaturated groups but also the cleavage of beta-O-4 bonds occurred. Stable products in thermal and chemical properties were formed, which possessed high heated value and low molecular weight. This treatment is conducive to suppressing the occurrence of condensation and favorable for the further catalytic conversion. |
| Subtype | Article |
| WOS Headings | Science & Technology ; Technology |
| DOI | 10.1021/acs.energyfuels.7b00934 |
| WOS Subject Extended | Energy & Fuels ; Engineering |
| WOS Keyword | HYDROGENOLYSIS PROCESS ; PHENOLIC-COMPOUNDS ; METAL CHLORIDE ; HYDRODEOXYGENATION ; CHEMICALS ; EFFICIENT ; VALORIZATION ; EVOLUTION ; ETHANOL ; MODEL |
| Indexed By | SCI |
| Language | 英语 |
| Funding Organization | Natural Science Foundation of China(51476178 ; Youth Science and Technology Innovation Talents of Guangdong Province(2015TQ01N652) ; Youth Innovation Promotion Association of Chinese Academy of Sciences(2016313) ; 51676191) |
| WOS Subject | Energy & Fuels ; Engineering, Chemical |
| WOS ID | WOS:000406356600058 |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/15757 |
| Collection | 中国科学院广州能源研究所 |
| Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 2.CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China 3.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
| Recommended Citation GB/T 7714 | Shu, Riyang,Xu, Ying,Chen, Pengru,et al. Mild Hydrogenation of Lignin Depolymerization Products Over Ni/SiO2 Catalyst[J]. ENERGY & FUELS,2017,31(7):7208-7213. |
| APA | Shu, Riyang.,Xu, Ying.,Chen, Pengru.,Ma, Longlong.,Zhang, Qi.,...&Wang, Chenguang.(2017).Mild Hydrogenation of Lignin Depolymerization Products Over Ni/SiO2 Catalyst.ENERGY & FUELS,31(7),7208-7213. |
| MLA | Shu, Riyang,et al."Mild Hydrogenation of Lignin Depolymerization Products Over Ni/SiO2 Catalyst".ENERGY & FUELS 31.7(2017):7208-7213. |
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