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In-situ hydrogenation of model compounds and raw bio-oil over Ni/CMK-3 catalyst
Xu, Ying1,2,3; Li, Yanbin1; Wang, Congwei1,2,3; Wang, Chenguang1,2,3; Ma, Longlong1,2,3; Wang, Tiejun1,2,3; Zhang, Xinghua1,2,3; Zhang, Qi1,2,3
2017-06-15
发表期刊FUEL PROCESSING TECHNOLOGY
卷号161页码:226-231
摘要Ni/CMK-3 catalyst, the mesoporous carbon material loading Ni activity, was prepared and used in the in-situ hydrogenation of mixed model compounds (including acetone, acetic acid, furfural, o-cresol, ethanediol and water) of bio-oil (MCB) and actual bio-oil in this paper. The effects of hydrogen donors, solvents and the dosages of catalyst were all investigated in the in-situ hydrogenation process. The results showed that the hydrogen donor of methanol, ethanol and formic acid could all provide hydrogen for the in-situ hydrogenation but the product distributions of bio-oils were different after in-situ hydrogenation. Using alcohols as hydrogen donors, esterification reaction happened between the hydrogen donors and acetic acid. The formic acid could promote the phenols conversion but the conversion of acetic acid was restrained. When the radio of water and methanol was 10:3 and 10:5, most of ketones and aldehydes in the raw bio-oil converted to alcohols and the conversion of acids and phenols was beyond 50%. The contents of alcohols and esters in raw bio-oil increased from 18.52% to 51.14% and 48.21%. (C) 2016 Elsevier B.V. All rights reserved.
文章类型Article
关键词Bio-oil In-situ Hydrogenation Model Compounds Ni-base Catalyst Cmk-3
WOS标题词Science & Technology ; Physical Sciences ; Technology
资助者Natural Science Foundation of China(51476178) ; Science and Technology Plan Key Project in Guangdong Province of China(2014A010106019) ; Youth Innovation Promotion Association CAS ; Natural Science Foundation of China(51476178) ; Science and Technology Plan Key Project in Guangdong Province of China(2014A010106019) ; Youth Innovation Promotion Association CAS
DOI10.1016/j.fuproc.2016.08.018
研究领域[WOS]Chemistry ; Energy & Fuels ; Engineering
关键词[WOS]FAST PYROLYSIS ; PHENOLIC-COMPOUNDS ; NI CATALYST ; HYDRODEOXYGENATION ; ESTERIFICATION ; CONVERSION ; CARBON ; HYDROCARBONS ; ALCOHOLS ; QUALITY
收录类别SCI
语种英语
资助者Natural Science Foundation of China(51476178) ; Science and Technology Plan Key Project in Guangdong Province of China(2014A010106019) ; Youth Innovation Promotion Association CAS ; Natural Science Foundation of China(51476178) ; Science and Technology Plan Key Project in Guangdong Province of China(2014A010106019) ; Youth Innovation Promotion Association CAS
WOS类目Chemistry, Applied ; Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000401047600027
引用统计
被引频次:5[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/14130
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
3.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
推荐引用方式
GB/T 7714
Xu, Ying,Li, Yanbin,Wang, Congwei,et al. In-situ hydrogenation of model compounds and raw bio-oil over Ni/CMK-3 catalyst[J]. FUEL PROCESSING TECHNOLOGY,2017,161:226-231.
APA Xu, Ying.,Li, Yanbin.,Wang, Congwei.,Wang, Chenguang.,Ma, Longlong.,...&Zhang, Qi.(2017).In-situ hydrogenation of model compounds and raw bio-oil over Ni/CMK-3 catalyst.FUEL PROCESSING TECHNOLOGY,161,226-231.
MLA Xu, Ying,et al."In-situ hydrogenation of model compounds and raw bio-oil over Ni/CMK-3 catalyst".FUEL PROCESSING TECHNOLOGY 161(2017):226-231.
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