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Conversion of Cellulose to 5-Hydroxymethylfurfural using Inorganic Acidic Catalysts in the Presence of Pressurized Water Steam
Cai, Chiliu1,2,3,4; Liu, Qiying1,2,3; Tan, Jin1,2,3; Wang, Tiejun1,2,3; Zhang, Qi1,2,3; Ma, Longlong1,2,3
2017
发表期刊BIORESOURCES
卷号12期号:1页码:1201-1215
摘要Traditionally, 5-hydroxymethylfurfural ( HMF) is produced by using a water-organic solvent medium, which inevitably increases production costs and adds subsequent separation processes. To minimize cost and/or toxic organic solvent usage, this study presents an effective pathway for producing HMF from cellulose. The process uses a fixed bed reactor with a steam stripping process in which the cellulose is converted into HMF and other products in the presence of acidic inorganic salts. In the process, the cellulose was hydrolyzed to glucose, which was followed by isomerization to fructose and fructose dehydration into HMF. The produced HMF was easily vaporized into the gas phase, which avoided its conversion into undesired byproducts. An acceptable HMF yield of 28.2 mol% was obtained using KH2PO4 as the catalyst at 270 degrees C. This technology could be used to obtain both HMF and furfural ( FF) from different lignocellulosic biomasses. This stripping technology has advantages such as the lack of organic solvents, showing an alternative and green HMF and/or FF production from lignocellulosic biomass.
文章类型Article
关键词Cellulose Hmf Conversion Steam Stripping Process Fixed Bed
WOS标题词Science & Technology ; Technology
资助者National Science Foundation of China(51536009 ; 51576199 ; 51376185) ; National Science Foundation of China(51536009 ; 51576199 ; 51376185)
DOI10.15376/biores.12.1.1201-1215
研究领域[WOS]Materials Science
关键词[WOS]LIQUID-WATER ; LEVULINIC ACID ; BIOMASS ; HYDROCARBONS ; HYDROLYSIS ; PRETREATMENT ; DEHYDRATION ; MECHANISM ; SOLVENTS ; ZEOLITE
收录类别SCI
语种英语
资助者National Science Foundation of China(51536009 ; 51576199 ; 51376185) ; National Science Foundation of China(51536009 ; 51576199 ; 51376185)
WOS类目Materials Science, Paper & Wood
WOS记录号WOS:000397065200088
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/14076
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
3.Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Cai, Chiliu,Liu, Qiying,Tan, Jin,et al. Conversion of Cellulose to 5-Hydroxymethylfurfural using Inorganic Acidic Catalysts in the Presence of Pressurized Water Steam[J]. BIORESOURCES,2017,12(1):1201-1215.
APA Cai, Chiliu,Liu, Qiying,Tan, Jin,Wang, Tiejun,Zhang, Qi,&Ma, Longlong.(2017).Conversion of Cellulose to 5-Hydroxymethylfurfural using Inorganic Acidic Catalysts in the Presence of Pressurized Water Steam.BIORESOURCES,12(1),1201-1215.
MLA Cai, Chiliu,et al."Conversion of Cellulose to 5-Hydroxymethylfurfural using Inorganic Acidic Catalysts in the Presence of Pressurized Water Steam".BIORESOURCES 12.1(2017):1201-1215.
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