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Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells
Bi, Zhuoneng1,2; Liang, Zhurong1,2; Xu, Xueqing1,2; Chai, Zhisheng1,2; Jin, Hu1,2; Xu, Dehua1,2; Li, Jingling1,2; Li, Minghua3; Xu, Gang1,2
2017-04-01
Source PublicationSOLAR ENERGY MATERIALS AND SOLAR CELLS
Volume162Pages:13-20
AbstractSpray deposition has been demonstrated to be a promising method to prepare perovskite thin film with many advantages, such as easy and processable under fully ambient condition, which is suitable for large-scale production. In this work, we reveal two typical spray deposition process of rapid and slow solvent evaporation. It is emphasized that the rapid solvent evaporation process is essential to avoid dendritic crystal and obtain dense perovskite thin film without pin-holes, which can be realized with a suitable substrate temperature. With optimized spray conditions including flow rate of precursor solution and carrier gas pressure, a dense and uniform perovskite layer with full surface coverage was immediately formed in similar to 5 s without any post-annealing process. The as-fabricated planar heterojunction solar cell achieved a power conversion efficiency (PCE) of 13.54% with 300 +/- 30 nm in thickness of perovskite layer. To the best of our knowledge, this result is the highest value for the CH3NH3PbI3 perovskite solar cells fabricated in air condition with high humidity up to 50%.
SubtypeArticle
KeywordCh3nh3pbi3 Perovskite Thin Film Spray Deposition Fast Preparation High Efficient Planar Solar Cells
WOS HeadingsScience & Technology ; Technology ; Physical Sciences
DOI10.1016/j.solmat2016.12.032
WOS Subject ExtendedEnergy & Fuels ; Materials Science ; Physics
WOS KeywordPERFORMANCE ; GROWTH ; CRYSTALLIZATION ; FABRICATION ; HYSTERESIS
Indexed BySCI
Language英语
Funding OrganizationNational Natural Science Foundation of China(21073193 ; Natural Science Foundation of Guangdong Province(2015A030310501) ; Project on the Collaborative Innovation and Environmental Construction Platform of Guangdong Province(2014A050503051) ; 21273241)
WOS SubjectEnergy & Fuels ; Materials Science, Multidisciplinary ; Physics, Applied
WOS IDWOS:000393720500003
Citation statistics
Cited Times:25[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/14048
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangdong Key Lab New & Renewable Energy Res & De, Key Lab Renewable Energy, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Guangdong Mech & Elect Polytech, Guangzhou 510515, Guangdong, Peoples R China
Recommended Citation
GB/T 7714
Bi, Zhuoneng,Liang, Zhurong,Xu, Xueqing,et al. Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells[J]. SOLAR ENERGY MATERIALS AND SOLAR CELLS,2017,162:13-20.
APA Bi, Zhuoneng.,Liang, Zhurong.,Xu, Xueqing.,Chai, Zhisheng.,Jin, Hu.,...&Xu, Gang.(2017).Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells.SOLAR ENERGY MATERIALS AND SOLAR CELLS,162,13-20.
MLA Bi, Zhuoneng,et al."Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells".SOLAR ENERGY MATERIALS AND SOLAR CELLS 162(2017):13-20.
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