GIEC OpenIR  > 中国科学院广州能源研究所
Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase
Chen, Lungang; Li, Yuping; Zhang, Xinghua; Zhang, Qi; Wang, Tiejun; Ma, Longlong
2017
Source PublicationCATALYSIS LETTERS
Volume147Issue:1Pages:29-38
AbstractThe aqueous-phase hydrogenation of propanoic acid was performed over the Ru/ZrO2 and Ru/Al2O3 catalysts with different Ru loading. Combined with multiple characterization techniques, such as H-2-TPR, XRD, CO-FTIR, and DRIFTS of propanoic acid, the effect of Ru loading on the decarbonylation/hydrogenation of propanoic acid was investigated. Although hydrogenation/decarbonylation of carboxylic acids were strongly affected by the nature of supports, the increase of metal loading can cause the larger Ru particles and more bare Ru metal sites, which can facilitate the C-C bond cleavage reaction derived from the decarbonylation of propanoyl species over Ru metal sites.
SubtypeArticle
KeywordRu Loading Carboxylic Acid Hydrogenation Decarbonylation C-c Cleavage
WOS HeadingsScience & Technology ; Physical Sciences
DOI10.1007/s10562-016-1877-4
WOS Subject ExtendedChemistry
WOS KeywordACETIC-ACID ; CO ADSORPTION ; LACTIC-ACID ; RUTHENIUM CATALYSTS ; SUCCINIC ACID ; HYDROGENATION ; BIOMASS ; HYDROGENOLYSIS ; REDUCTION ; CHEMICALS
Indexed BySCI
Language英语
Funding OrganizationNational Natural Science Foundation of China(51306189) ; Science and Technology Program of Guangdong Province(2014A010106022) ; Comprehensive Strategic Cooperation Project of Guangdong Province ; Chinese Academy of Sciences(2012B090400042) ; China-EU SMEs Cooperation Fund for Energy Conservation Research Project(SQ2013ZOB000002)
WOS SubjectChemistry, Physical
WOS IDWOS:000394139200004
Citation statistics
Cited Times:3[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/14037
Collection中国科学院广州能源研究所
AffiliationChinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
Recommended Citation
GB/T 7714
Chen, Lungang,Li, Yuping,Zhang, Xinghua,et al. Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase[J]. CATALYSIS LETTERS,2017,147(1):29-38.
APA Chen, Lungang,Li, Yuping,Zhang, Xinghua,Zhang, Qi,Wang, Tiejun,&Ma, Longlong.(2017).Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase.CATALYSIS LETTERS,147(1),29-38.
MLA Chen, Lungang,et al."Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase".CATALYSIS LETTERS 147.1(2017):29-38.
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