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Hydrodeoxygenation of Anisole over Ni/alpha-Al2O3 Catalyst
Tang, Wen-wu1,3; Zhang, Xing-hua2,3; Zhang, Qi2,3; Wang, Tie-jun2,3; Ma, Long-long2,3
2016-10-01
发表期刊CHINESE JOURNAL OF CHEMICAL PHYSICS
卷号29期号:5页码:617-622
摘要Ni-based catalysts supported on different supports (alpha-Al2O3, gamma-Al2O3, SiO2, TiO2, and ZrO2) were prepared by impregnation. Effects of supports on catalytic performance were tested using hydrodeoxygenation reaction (HDO) of anisole as model reaction. Ni/alpha-Al2O3 was found to be the highest active catalyst for HDO of anisole. Under the optimal conditions, the anisole conversion is 93.25% and the hydrocarbon yield is 90.47%. Catalyst characterization using H-2-TPD method demonstrates that Ni/alpha-Al2O3 catalyst possesses more amount of active metal Ni than those of other investigated catalysts, which can enhance the catalytic activity for hydrogenation. Furthermore, it is found that the Ni/alpha-Al2O3 catalyst has excellent repeatability, and the carbon deposited on the surface of catalyst is negligible.
文章类型Article
关键词Anisole Hydrodeoxygenation Ni/alpha-al2o3 Hydrocarbons
WOS标题词Science & Technology ; Physical Sciences
资助者National Natural Science Foundation of China(51576198) ; National Key Technology RD Program(2014BAD02B01) ; Youth Innovation Promotion Association of Chinese Academy of Sciences(2015288) ; National Natural Science Foundation of China(51576198) ; National Key Technology RD Program(2014BAD02B01) ; Youth Innovation Promotion Association of Chinese Academy of Sciences(2015288)
DOI10.1063/1674-0068/29/cjcp1603062
研究领域[WOS]Physics
关键词[WOS]LIGNIN DEPOLYMERIZATION ; PHENOLIC-COMPOUNDS ; AQUEOUS-PHASE ; BIO-OIL ; EFFICIENT ; GUAIACOL ; DECOMPOSITION ; HYDROCARBONS ; VALORIZATION ; CONVERSION
收录类别SCI
语种英语
资助者National Natural Science Foundation of China(51576198) ; National Key Technology RD Program(2014BAD02B01) ; Youth Innovation Promotion Association of Chinese Academy of Sciences(2015288) ; National Natural Science Foundation of China(51576198) ; National Key Technology RD Program(2014BAD02B01) ; Youth Innovation Promotion Association of Chinese Academy of Sciences(2015288)
WOS类目Physics, Atomic, Molecular & Chemical
WOS记录号WOS:000388063400015
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/13975
专题中国科学院广州能源研究所
作者单位1.Univ Sci & Technol China, Dept Chem, Hefei 230026, Peoples R China
2.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
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Tang, Wen-wu,Zhang, Xing-hua,Zhang, Qi,et al. Hydrodeoxygenation of Anisole over Ni/alpha-Al2O3 Catalyst[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2016,29(5):617-622.
APA Tang, Wen-wu,Zhang, Xing-hua,Zhang, Qi,Wang, Tie-jun,&Ma, Long-long.(2016).Hydrodeoxygenation of Anisole over Ni/alpha-Al2O3 Catalyst.CHINESE JOURNAL OF CHEMICAL PHYSICS,29(5),617-622.
MLA Tang, Wen-wu,et al."Hydrodeoxygenation of Anisole over Ni/alpha-Al2O3 Catalyst".CHINESE JOURNAL OF CHEMICAL PHYSICS 29.5(2016):617-622.
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