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Jet-Fuel Range Hydrocarbons from Biomass-Derived Sorbitol over Ni-HZSM-5/SBA-15 Catalyst
Weng, Yujing1,2; Qiu, Songbai1; Ma, Longlong1; Liu, Qiying1; Ding, Mingyue1; Zhang, Qian1,2; Zhang, Qi1; Wang, Tiejun1
2015-12-01
发表期刊CATALYSTS
卷号5期号:4页码:2147-2160
摘要Aromatics and cyclic-hydrocarbons are the significant components of jet fuel with high energy-density. However, conventional technologies for bio-fuel production cannot produce these products without further aromatization and isomerization. In this work, renewable liquid fuel with high content of aromatics and cyclic-hydrocarbons was obtained through aqueous catalytic conversion of biomass sorbitol over Ni-HZSM-5/SBA-15 catalyst. Texture characteristics of the catalyst were determined by physisorption of N-2, which indicated its bimodal pore structures were microporous (HZSM-5, pore width: 0.56 nm) and mesoporous (SBA-15, pore width: 8 nm). The surface acidity included weak and strong acid sites, predominantly Lewis type, and was further confirmed by the NH3-TPD and Py-IR analysis. The catalytic performances were tested in a fixed-bed reactor under the conditions of 593 K, WHSV of 0.75 h(-1), GHSV of 2500 h(-1) and 4.0 MPa of hydrogen pressure, whereby oil yield of 40.4 wt. % with aromatics and cyclic-hydrocarbons content of 80.0% was obtained.
文章类型Article
关键词Sorbitol Aromatic Cyclic-hydrocarbon Long-chain Alkane Aqueous Catalysis
WOS标题词Science & Technology ; Physical Sciences
DOI10.3390/catal5042147
研究领域[WOS]Chemistry
关键词[WOS]NI/HZSM-5 CATALYSTS ; PRODUCT DISTRIBUTION ; CO-IMPREGNATION ; ALKYL-AROMATICS ; CONVERSION ; TRANSFORMATION ; GASOLINE ; GLYCEROL ; METHANOL ; ZEOLITE
收录类别SCI
语种英语
WOS类目Chemistry, Physical
WOS记录号WOS:000367535300034
引用统计
被引频次:12[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10939
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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Weng, Yujing,Qiu, Songbai,Ma, Longlong,et al. Jet-Fuel Range Hydrocarbons from Biomass-Derived Sorbitol over Ni-HZSM-5/SBA-15 Catalyst[J]. CATALYSTS,2015,5(4):2147-2160.
APA Weng, Yujing.,Qiu, Songbai.,Ma, Longlong.,Liu, Qiying.,Ding, Mingyue.,...&Wang, Tiejun.(2015).Jet-Fuel Range Hydrocarbons from Biomass-Derived Sorbitol over Ni-HZSM-5/SBA-15 Catalyst.CATALYSTS,5(4),2147-2160.
MLA Weng, Yujing,et al."Jet-Fuel Range Hydrocarbons from Biomass-Derived Sorbitol over Ni-HZSM-5/SBA-15 Catalyst".CATALYSTS 5.4(2015):2147-2160.
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