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Laser Raman Spectroscopy and Its Application in Gas Hydrate Studies
Fu Juan1,2,5; Wu Neng-you2,4; Lu Hai-long3; Wu Dai-dai2; Su Qiu-cheng2
2015-11-01
Source PublicationSPECTROSCOPY AND SPECTRAL ANALYSIS
Volume35Issue:11
AbstractGas hydrates are important potential energy resources. Microstructural characterization of gas hydrate can provide information to study the mechanism of gas hydrate formation and to support the exploitation and application of gas hydrate technology. This article systemly introduces the basic principle of laser Raman spectroscopy and summarizes its application in gas hydrate studies. Based on Raman results, not only can the information about gas composition and structural type be deduced, but also the occupancies of large and small cages and even hydration number can be calculated from the relative intensities of Raman peaks. By using the in-situ analytical technology, laser Raman specstropy can be applied to characterize the formation and decomposition processes of gas hydrate at microscale, for example the enclathration and leaving of gas molecules into/from its cages, to monitor the changes in gas concentration and gas solubility during hydrate formation and decomposition, and to identify phase changes in the study system. Laser Raman in-situ analytical technology has also been used in determination of hydrate structure and understanding its changing process under the conditions of ultra high pressure. Deep-sea in-situ Raman spectrometer can be employed for the in-situ analysis of the structures of natural gas hydrate and their formation environment. Raman imaging technology can be applied to specify the characteristics of crystallization and gas distribution over hydrate surface. With the development of laser Raman technology and its combination with other instruments, it will become more powerful and play a more significant role in the microscopic study of gas hydrate.
SubtypeArticle
KeywordLaser Raman Gas Hydrate In-situ Analysis Raman Imaging
WOS HeadingsScience & Technology ; Technology
DOI10.3964/j.issn.1000-0593(2015)11-2996-07
WOS Subject ExtendedSpectroscopy
WOS KeywordMETHANE HYDRATE ; OCEAN ; DISSOCIATION ; NUMBER ; WATER
Indexed BySCI
Language英语
WOS SubjectSpectroscopy
WOS IDWOS:000364503600004
Citation statistics
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10898
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Geochem, Guangzhou 510640, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
3.Peking Univ, Coll Engn, Beijing 100871, Peoples R China
4.Qingdao Inst Marine Geol, Qingdao 266071, Peoples R China
5.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Fu Juan,Wu Neng-you,Lu Hai-long,et al. Laser Raman Spectroscopy and Its Application in Gas Hydrate Studies[J]. SPECTROSCOPY AND SPECTRAL ANALYSIS,2015,35(11).
APA Fu Juan,Wu Neng-you,Lu Hai-long,Wu Dai-dai,&Su Qiu-cheng.(2015).Laser Raman Spectroscopy and Its Application in Gas Hydrate Studies.SPECTROSCOPY AND SPECTRAL ANALYSIS,35(11).
MLA Fu Juan,et al."Laser Raman Spectroscopy and Its Application in Gas Hydrate Studies".SPECTROSCOPY AND SPECTRAL ANALYSIS 35.11(2015).
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