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Efficient valorization of lignin depolymerization products in the present of NixMg1-xO
Long, Jinxing; Shu, Riyang; Yuan, Zhengqiu; Wang, Tiejun; Xu, Ying; Zhang, Xinghua; Zhang, Qi; Ma, Longlong
2015-11-01
发表期刊APPLIED ENERGY
卷号157
摘要Efficient conversion of lignin depolymerization products to more stable chemicals has attracted increasing attention during last few years. Here, we reported a novel and efficient method for lignin depolymerization products valorization on the simple and economic catalyst NixMg1-xO. In which, the unsaturated ingredients were converted to thermal and chemical stable products, resulting in the obvious decreasing of the unsaturated degree of the products and the repolymerization of the phenolic oligomer. The results showed that more than 98% of phenol, a model chemical of lignin depolymerization products, could be converted to cyclohexanol with 100% selectivity. Further investigation demonstrated that it was also efficient for the real lignin depolymerization products, where a significant decrease on the oxygen content and the average molecular weight were shown. Moreover, the NixMg1-xO catalyst was recyclable, and no significant loss of the catalytic activity was exhibited even after 5 runs. (C) 2015 Elsevier Ltd. All rights reserved.
文章类型Article
关键词Lignin Depolymerization Products Phenol Nixmg1-xo Recyclability Cyclohexanol
WOS标题词Science & Technology ; Technology
DOI10.1016/j.apenergy.2015.04.011
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]ACIDIC IONIC LIQUIDS ; CATALYTIC CONVERSION ; BIOMASS GASIFICATION ; ORGANOSOLV LIGNIN ; BIO-OIL ; HYDRODEOXYGENATION ; PYROLYSIS ; CHEMICALS ; BAGASSE ; NMR
收录类别SCI
语种英语
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000364249200054
引用统计
被引频次:14[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10886
专题中国科学院广州能源研究所
作者单位Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
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GB/T 7714
Long, Jinxing,Shu, Riyang,Yuan, Zhengqiu,et al. Efficient valorization of lignin depolymerization products in the present of NixMg1-xO[J]. APPLIED ENERGY,2015,157.
APA Long, Jinxing.,Shu, Riyang.,Yuan, Zhengqiu.,Wang, Tiejun.,Xu, Ying.,...&Ma, Longlong.(2015).Efficient valorization of lignin depolymerization products in the present of NixMg1-xO.APPLIED ENERGY,157.
MLA Long, Jinxing,et al."Efficient valorization of lignin depolymerization products in the present of NixMg1-xO".APPLIED ENERGY 157(2015).
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