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Study on Pilot-Scale CO2 Separation from Flue Gas by the Hydrate Method
Xu, Chun-Gang1,2; Chen, Zhao-Yang1,2; Cai, Jing1,2; Li, Xiao-Sen1,2
2014-02-01
发表期刊ENERGY & FUELS
卷号28期号:2页码:1242-1248
摘要Technology of hydrate-based CO2 separation and capture is considered as a green and economical gas separation technology and is extensively studied. Most of the previous studies involving the aspects of thermodynamics and kinetics of the CO2 gas hydrate formation were carried out with small reactors, whereas few studies were carried out with pilot-scale equipments. In this paper, a pilot-scale CO2 separation from flue gas by the hydrate method is reported. By the equipment, we successfully realize CO2 separation from flue gas. By a two-stage hydrate separation process, the CO2 concentration can be enhanced to approximately 90.0% from 17.0%. The effects of the operating pressure and gas flow rate on CO2 recovery are also investigated by comparing and analyzing the data of the CO2 concentration, gas consumption, and CO2 recovery. The higher pressure results in the higher CO2 recovery, and there is an optimal ratio of the gas flow rate to the fluid flow rate for obtaining the highest gas consumption. The results achieved in this paper will be an important foundation to further develop the continuous CO2 hydrate separation process.
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/ef401883v
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]CARBON-DIOXIDE CAPTURE ; PRE-COMBUSTION CAPTURE ; FIXED-BED REACTOR ; CYCLOPENTANE ; MIXTURES ; TETRAHYDROFURAN
收录类别SCI
语种英语
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000331861800059
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10674
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
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GB/T 7714
Xu, Chun-Gang,Chen, Zhao-Yang,Cai, Jing,et al. Study on Pilot-Scale CO2 Separation from Flue Gas by the Hydrate Method[J]. ENERGY & FUELS,2014,28(2):1242-1248.
APA Xu, Chun-Gang,Chen, Zhao-Yang,Cai, Jing,&Li, Xiao-Sen.(2014).Study on Pilot-Scale CO2 Separation from Flue Gas by the Hydrate Method.ENERGY & FUELS,28(2),1242-1248.
MLA Xu, Chun-Gang,et al."Study on Pilot-Scale CO2 Separation from Flue Gas by the Hydrate Method".ENERGY & FUELS 28.2(2014):1242-1248.
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