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Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor
Lv, Qiu-Nan; Li, Xiao-Sen1; Xu, Chun-Gang; Chen, Zhao-Yang
2012-05-02
发表期刊INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷号51期号:17页码:5967-5975
摘要The effects of the flow rates of cyclopentane (CP) and methane gas, operating pressure, and experimental temperature on the formation of c-yclopentane-methane hydrate were investigated using a novel bubble column reactor. The results indicated that, with either an increase of the operating pressure or a decrease of the experimental temperature, the induction time decreased whereas the cumulative gas consumption and gas conversion ratio increased. In addition, with an increase of the flow rate of methane gas, the induction time decreased, whereas the cumulative gas consumption increased. The gas conversion ratio increased first from 61.5% to 93.1% when the flow rate of methane gas increased from 159 to 234 mL/min and then decreased from 93.1% to 83.2% when the flow rate of methane gas continuously increased from 234 mL/min to 308.9 mL/min. This decrease was attributed to an increase of the discharge rate of methane from the reactor. It was noted the average methane consumption rate could be effectively enhanced with an increase of the flow rate of gas at relatively low pressure and high temperature. The flow rate of CP had a minimal effect on the cumulative gas consumption and gas conversion ratio. However, an increase of the flow rate of CP could reduce the induction time.
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/ie202422c
研究领域[WOS]Engineering
关键词[WOS]GAS HYDRATE ; CARBON-DIOXIDE ; CAPTURE ; CO2 ; WATER
收录类别SCI
语种英语
WOS类目Engineering, Chemical
WOS记录号WOS:000303370000017
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10568
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
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GB/T 7714
Lv, Qiu-Nan,Li, Xiao-Sen,Xu, Chun-Gang,et al. Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2012,51(17):5967-5975.
APA Lv, Qiu-Nan,Li, Xiao-Sen,Xu, Chun-Gang,&Chen, Zhao-Yang.(2012).Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,51(17),5967-5975.
MLA Lv, Qiu-Nan,et al."Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 51.17(2012):5967-5975.
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