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Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor
Lv, Qiu-Nan; Li, Xiao-Sen1; Xu, Chun-Gang; Chen, Zhao-Yang
2012-05-02
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume51Issue:17Pages:5967-5975
AbstractThe effects of the flow rates of cyclopentane (CP) and methane gas, operating pressure, and experimental temperature on the formation of c-yclopentane-methane hydrate were investigated using a novel bubble column reactor. The results indicated that, with either an increase of the operating pressure or a decrease of the experimental temperature, the induction time decreased whereas the cumulative gas consumption and gas conversion ratio increased. In addition, with an increase of the flow rate of methane gas, the induction time decreased, whereas the cumulative gas consumption increased. The gas conversion ratio increased first from 61.5% to 93.1% when the flow rate of methane gas increased from 159 to 234 mL/min and then decreased from 93.1% to 83.2% when the flow rate of methane gas continuously increased from 234 mL/min to 308.9 mL/min. This decrease was attributed to an increase of the discharge rate of methane from the reactor. It was noted the average methane consumption rate could be effectively enhanced with an increase of the flow rate of gas at relatively low pressure and high temperature. The flow rate of CP had a minimal effect on the cumulative gas consumption and gas conversion ratio. However, an increase of the flow rate of CP could reduce the induction time.
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
DOI10.1021/ie202422c
WOS Subject ExtendedEngineering
WOS KeywordGAS HYDRATE ; CARBON-DIOXIDE ; CAPTURE ; CO2 ; WATER
Indexed BySCI
Language英语
WOS SubjectEngineering, Chemical
WOS IDWOS:000303370000017
Citation statistics
Cited Times:24[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10568
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
Recommended Citation
GB/T 7714
Lv, Qiu-Nan,Li, Xiao-Sen,Xu, Chun-Gang,et al. Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2012,51(17):5967-5975.
APA Lv, Qiu-Nan,Li, Xiao-Sen,Xu, Chun-Gang,&Chen, Zhao-Yang.(2012).Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,51(17),5967-5975.
MLA Lv, Qiu-Nan,et al."Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 51.17(2012):5967-5975.
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