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Characteristics of biomass gasification using chemical looping with iron ore as an oxygen carrier
Huang, Zhen1; He, Fang1; Feng, Yipeng1; Liu, Rundong2; Zhao, Kun1; Zheng, Anqing1; Chang, Sheng1; Zhao, Zengli1; Li, Haibin1
2013-11-13
发表期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷号38期号:34页码:14568-14575
摘要Experiments regarding to biomass gasification using chemical looping (BGCL) were carried out in a fluidized bed reactor under argon atmosphere. Iron ore (natural hematite) was used as an oxygen carrier in the study. Similar to steam, a performance of oxygen carrier which provided oxygen source for biomass gasification by acting as a gasifying medium was found. An optimum Fe2O3/C molar ratio of 0.23 was determined with the aim of obtaining maximum gas yield of 1.06 Nm(3)/kg and gasification efficiency of 83.31%. The oxygen carrier was gradually deactivated with reduction time increasing, inhibiting the carbon and hydrogen in biomass from being converted into synthesis gas. The fraction of Fe2+ increased from 0 to 47.12% after reduction time of 45 min, which implied that active lattice oxygen of 49.75% was consumed. The oxygen carrier of fresh and reacted was analyzed by a series of characterization methods, such as X-ray diffraction (XRD), Scanning electron microscopy (SEM), and Energy-dispersive X-ray spectroscopy (EDX). Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
文章类型Article
关键词Biomass Gasification Chemical Looping Lattice Oxygen Iron Ore
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.ijhydene.2013.09.022
研究领域[WOS]Chemistry ; Electrochemistry ; Energy & Fuels
关键词[WOS]SYNTHESIS GAS-PRODUCTION ; FLUIDIZED-BED ; COMBUSTION ; COAL ; FE ; OXIDE ; CONVERSION ; MINERALS ; REACTOR ; SCALE
收录类别SCI
语种英语
WOS类目Chemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS记录号WOS:000328517700021
引用统计
被引频次:26[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10105
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Univ Toledo, Dept Environm Sci, Toledo, OH 43606 USA
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Huang, Zhen,He, Fang,Feng, Yipeng,et al. Characteristics of biomass gasification using chemical looping with iron ore as an oxygen carrier[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2013,38(34):14568-14575.
APA Huang, Zhen.,He, Fang.,Feng, Yipeng.,Liu, Rundong.,Zhao, Kun.,...&Li, Haibin.(2013).Characteristics of biomass gasification using chemical looping with iron ore as an oxygen carrier.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,38(34),14568-14575.
MLA Huang, Zhen,et al."Characteristics of biomass gasification using chemical looping with iron ore as an oxygen carrier".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 38.34(2013):14568-14575.
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