Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge

doi:10.1016/j.apenergy.2012.12.017

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	Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge
	Ding, Mingyue1 ; Hayakawa, Taichi 2; Zeng, Chunyang 2; Jin, Yuzhou 2; Zhang, Qi1 ; Wang, Tiejun1 ; Ma, Longlong1 ; Yoneyama, Yoshiharu 2; Tsubaki, Noritatsu 2,3
	2013-04-01
发表期刊	APPLIED ENERGY
卷号	104 页码:777-782
摘要	Non-catalytic direct conversion of liquid natural gas (LNG) to syngas and ethylene using pulse discharge technology was firstly carried out under the temperature of liquid nitrogen and atmospheric pressure. The liquefaction of natural gas increased tremendously the collision frequency between electrons and methane molecules in the discharge region and promoted the dimerisation of CH2 radicals formed, inducing the formation of large amounts of ethylene (selectivity > 90%) and synthesis gas, and suppressing the proceeding of useless side-reactions. Especially, CO2 formation was suppressed remarkably due to the very low temperature of LNG and the cage effect provided by the condensed LNG. Crown Copyright (C) 2012 Published by Elsevier Ltd. All rights reserved.
文章类型	Article
关键词	Liquid Natural Gas Pulse Discharge Technology Cage Effect Syngas And Ethylene
WOS标题词	Science & Technology ; Technology
DOI	10.1016/j.apenergy.2012.12.017
研究领域[WOS]	Energy & Fuels ; Engineering
关键词[WOS]	CATALYTIC PARTIAL-OXIDATION ; LOW-TEMPERATURE PLASMA ; METHANE CONVERSION ; ATMOSPHERIC-PRESSURE ; ROOM-TEMPERATURE ; ACETYLENE ; ACTIVATION
收录类别	SCI
语种	英语
WOS类目	Energy & Fuels ; Engineering, Chemical
WOS记录号	WOS:000316152700075
引用统计	被引频次：11[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/10036
专题	中国科学院广州能源研究所
作者单位	1.Chinese Acad Sci, Key Lab Renewable Energy & Gas Hydrate, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 2.Toyama Univ, Dept Appl Chem, Sch Engn, Toyama 9308555, Japan 3.Japan Sci & Technol Agcy JST, ACT C, Tokyo 1028666, Japan
推荐引用方式 GB/T 7714	Ding, Mingyue,Hayakawa, Taichi,Zeng, Chunyang,et al. Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge[J]. APPLIED ENERGY,2013,104:777-782.
APA	Ding, Mingyue.,Hayakawa, Taichi.,Zeng, Chunyang.,Jin, Yuzhou.,Zhang, Qi.,...&Tsubaki, Noritatsu.(2013).Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge.APPLIED ENERGY,104,777-782.
MLA	Ding, Mingyue,et al."Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge".APPLIED ENERGY 104(2013):777-782.