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Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge
Ding, Mingyue1; Hayakawa, Taichi2; Zeng, Chunyang2; Jin, Yuzhou2; Zhang, Qi1; Wang, Tiejun1; Ma, Longlong1; Yoneyama, Yoshiharu2; Tsubaki, Noritatsu2,3
2013-04-01
发表期刊APPLIED ENERGY
卷号104页码:777-782
摘要Non-catalytic direct conversion of liquid natural gas (LNG) to syngas and ethylene using pulse discharge technology was firstly carried out under the temperature of liquid nitrogen and atmospheric pressure. The liquefaction of natural gas increased tremendously the collision frequency between electrons and methane molecules in the discharge region and promoted the dimerisation of CH2 radicals formed, inducing the formation of large amounts of ethylene (selectivity > 90%) and synthesis gas, and suppressing the proceeding of useless side-reactions. Especially, CO2 formation was suppressed remarkably due to the very low temperature of LNG and the cage effect provided by the condensed LNG. Crown Copyright (C) 2012 Published by Elsevier Ltd. All rights reserved.
文章类型Article
关键词Liquid Natural Gas Pulse Discharge Technology Cage Effect Syngas And Ethylene
WOS标题词Science & Technology ; Technology
DOI10.1016/j.apenergy.2012.12.017
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]CATALYTIC PARTIAL-OXIDATION ; LOW-TEMPERATURE PLASMA ; METHANE CONVERSION ; ATMOSPHERIC-PRESSURE ; ROOM-TEMPERATURE ; ACETYLENE ; ACTIVATION
收录类别SCI
语种英语
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000316152700075
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10036
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Key Lab Renewable Energy & Gas Hydrate, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Toyama Univ, Dept Appl Chem, Sch Engn, Toyama 9308555, Japan
3.Japan Sci & Technol Agcy JST, ACT C, Tokyo 1028666, Japan
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Ding, Mingyue,Hayakawa, Taichi,Zeng, Chunyang,et al. Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge[J]. APPLIED ENERGY,2013,104:777-782.
APA Ding, Mingyue.,Hayakawa, Taichi.,Zeng, Chunyang.,Jin, Yuzhou.,Zhang, Qi.,...&Tsubaki, Noritatsu.(2013).Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge.APPLIED ENERGY,104,777-782.
MLA Ding, Mingyue,et al."Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge".APPLIED ENERGY 104(2013):777-782.
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