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Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge
Ding, Mingyue1; Hayakawa, Taichi2; Zeng, Chunyang2; Jin, Yuzhou2; Zhang, Qi1; Wang, Tiejun1; Ma, Longlong1; Yoneyama, Yoshiharu2; Tsubaki, Noritatsu2,3
2013-04-01
Source PublicationAPPLIED ENERGY
Volume104Pages:777-782
AbstractNon-catalytic direct conversion of liquid natural gas (LNG) to syngas and ethylene using pulse discharge technology was firstly carried out under the temperature of liquid nitrogen and atmospheric pressure. The liquefaction of natural gas increased tremendously the collision frequency between electrons and methane molecules in the discharge region and promoted the dimerisation of CH2 radicals formed, inducing the formation of large amounts of ethylene (selectivity > 90%) and synthesis gas, and suppressing the proceeding of useless side-reactions. Especially, CO2 formation was suppressed remarkably due to the very low temperature of LNG and the cage effect provided by the condensed LNG. Crown Copyright (C) 2012 Published by Elsevier Ltd. All rights reserved.
SubtypeArticle
KeywordLiquid Natural Gas Pulse Discharge Technology Cage Effect Syngas And Ethylene
WOS HeadingsScience & Technology ; Technology
DOI10.1016/j.apenergy.2012.12.017
WOS Subject ExtendedEnergy & Fuels ; Engineering
WOS KeywordCATALYTIC PARTIAL-OXIDATION ; LOW-TEMPERATURE PLASMA ; METHANE CONVERSION ; ATMOSPHERIC-PRESSURE ; ROOM-TEMPERATURE ; ACETYLENE ; ACTIVATION
Indexed BySCI
Language英语
WOS SubjectEnergy & Fuels ; Engineering, Chemical
WOS IDWOS:000316152700075
Citation statistics
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10036
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Key Lab Renewable Energy & Gas Hydrate, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Toyama Univ, Dept Appl Chem, Sch Engn, Toyama 9308555, Japan
3.Japan Sci & Technol Agcy JST, ACT C, Tokyo 1028666, Japan
Recommended Citation
GB/T 7714
Ding, Mingyue,Hayakawa, Taichi,Zeng, Chunyang,et al. Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge[J]. APPLIED ENERGY,2013,104:777-782.
APA Ding, Mingyue.,Hayakawa, Taichi.,Zeng, Chunyang.,Jin, Yuzhou.,Zhang, Qi.,...&Tsubaki, Noritatsu.(2013).Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge.APPLIED ENERGY,104,777-782.
MLA Ding, Mingyue,et al."Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge".APPLIED ENERGY 104(2013):777-782.
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