Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts | |
Yan, Chang-Feng1,2; Cheng, Fei-Fei1,2; Hu, Rong-Rong1 | |
2010-11-01 | |
发表期刊 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY |
ISSN | 0360-3199 |
卷号 | 35期号:21页码:11693-11699 |
产权排序 | [Yan, Chang-Feng; Cheng, Fei-Fei; Hu, Rong-Rong] Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China; [Yan, Chang-Feng; Cheng, Fei-Fei] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China |
通讯作者 | yancf@ms.giec.ac.cn |
摘要 | A series of composite catalysts Ni/CeO2-ZrO2 were prepared via impregnation method with Ni as the active metal. A laboratory-scale fixed-bed reactor was employed to investigate the catalyst performance during hydrogen production by steam reforming bio-oil aqueous fraction. Effects of water-to-bio-oil ratio (W/B), reaction temperature, and the loaded weight of Ni and Ce on the hydrogen production performance of Nil CeO2-ZrO2 catalysts were examined. The obtained results were compared with commercial nickel-based catalysts (Z417). The best performance of Ni/CeO2-ZrO2 catalyst was observed when the Ni and Ce loaded weight were 12% and 7.5% respectively. At W/B = 4.9, T = 800 degrees C, H-2 yield reaches the highest of 69.7% and H-2 content of 61.8% were obtained. Under the same condition, H-2 yield and H-2 content were higher than commercial nickel-based catalysts (Z417). (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved. |
文章类型 | Article |
其他摘要 | A series of composite catalysts Ni/CeO2-ZrO2 were prepared via impregnation method with Ni as the active metal. A laboratory-scale fixed-bed reactor was employed to investigate the catalyst performance during hydrogen production by steam reforming bio-oil aqueous fraction. Effects of water-to-bio-oil ratio (W/B), reaction temperature, and the loaded weight of Ni and Ce on the hydrogen production performance of Nil CeO2-ZrO2 catalysts were examined. The obtained results were compared with commercial nickel-based catalysts (Z417). The best performance of Ni/CeO2-ZrO2 catalyst was observed when the Ni and Ce loaded weight were 12% and 7.5% respectively. At W/B = 4.9, T = 800 degrees C, H-2 yield reaches the highest of 69.7% and H-2 content of 61.8% were obtained. Under the same condition, H-2 yield and H-2 content were higher than commercial nickel-based catalysts (Z417). (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved. |
关键词 | Ni/ceo2-zro2 Hydrogen Bio-oil Steam Reforming |
学科领域 | Chemistry ; Electrochemistry ; Energy & Fuels |
WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
DOI | 10.1016/j.ijhydene.2010.08.083 |
研究领域[WOS] | Chemistry ; Electrochemistry ; Energy & Fuels |
URL | 查看原文 |
关键词[WOS] | ACETIC-ACID ; FAST-PYROLYSIS ; BIOMASS PYROLYSIS ; NICKEL-CATALYSTS ; METAL-CATALYSTS ; MODEL COMPOUNDS ; BED REACTOR ; TEMPERATURE ; ETHANOL ; GASIFICATION |
收录类别 | SCI |
语种 | 英语 |
项目资助者 | Natural Science Foundation of China [20806082, 50306026] |
WOS类目 | Chemistry, Physical ; Electrochemistry ; Energy & Fuels |
WOS记录号 | WOS:000283959900004 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.giec.ac.cn/handle/344007/8479 |
专题 | 中国科学院广州能源研究所 |
作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Yan, Chang-Feng,Cheng, Fei-Fei,Hu, Rong-Rong. Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2010,35(21):11693-11699. |
APA | Yan, Chang-Feng,Cheng, Fei-Fei,&Hu, Rong-Rong.(2010).Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,35(21),11693-11699. |
MLA | Yan, Chang-Feng,et al."Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 35.21(2010):11693-11699. |
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