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Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts
Yan, Chang-Feng1,2; Cheng, Fei-Fei1,2; Hu, Rong-Rong1
2010-11-01
Source PublicationINTERNATIONAL JOURNAL OF HYDROGEN ENERGY
ISSN0360-3199
Volume35Issue:21Pages:11693-11699
Contribution Rank[Yan, Chang-Feng; Cheng, Fei-Fei; Hu, Rong-Rong] Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China; [Yan, Chang-Feng; Cheng, Fei-Fei] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
Corresponding Authoryancf@ms.giec.ac.cn
AbstractA series of composite catalysts Ni/CeO2-ZrO2 were prepared via impregnation method with Ni as the active metal. A laboratory-scale fixed-bed reactor was employed to investigate the catalyst performance during hydrogen production by steam reforming bio-oil aqueous fraction. Effects of water-to-bio-oil ratio (W/B), reaction temperature, and the loaded weight of Ni and Ce on the hydrogen production performance of Nil CeO2-ZrO2 catalysts were examined. The obtained results were compared with commercial nickel-based catalysts (Z417). The best performance of Ni/CeO2-ZrO2 catalyst was observed when the Ni and Ce loaded weight were 12% and 7.5% respectively. At W/B = 4.9, T = 800 degrees C, H-2 yield reaches the highest of 69.7% and H-2 content of 61.8% were obtained. Under the same condition, H-2 yield and H-2 content were higher than commercial nickel-based catalysts (Z417). (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
SubtypeArticle
Other AbstractA series of composite catalysts Ni/CeO2-ZrO2 were prepared via impregnation method with Ni as the active metal. A laboratory-scale fixed-bed reactor was employed to investigate the catalyst performance during hydrogen production by steam reforming bio-oil aqueous fraction. Effects of water-to-bio-oil ratio (W/B), reaction temperature, and the loaded weight of Ni and Ce on the hydrogen production performance of Nil CeO2-ZrO2 catalysts were examined. The obtained results were compared with commercial nickel-based catalysts (Z417). The best performance of Ni/CeO2-ZrO2 catalyst was observed when the Ni and Ce loaded weight were 12% and 7.5% respectively. At W/B = 4.9, T = 800 degrees C, H-2 yield reaches the highest of 69.7% and H-2 content of 61.8% were obtained. Under the same condition, H-2 yield and H-2 content were higher than commercial nickel-based catalysts (Z417). (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
KeywordNi/ceo2-zro2 Hydrogen Bio-oil Steam Reforming
Subject AreaChemistry ; Electrochemistry ; Energy & Fuels
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1016/j.ijhydene.2010.08.083
WOS Subject ExtendedChemistry ; Electrochemistry ; Energy & Fuels
URL查看原文
WOS KeywordACETIC-ACID ; FAST-PYROLYSIS ; BIOMASS PYROLYSIS ; NICKEL-CATALYSTS ; METAL-CATALYSTS ; MODEL COMPOUNDS ; BED REACTOR ; TEMPERATURE ; ETHANOL ; GASIFICATION
Indexed BySCI
Language英语
Funding OrganizationNatural Science Foundation of China [20806082, 50306026]
WOS SubjectChemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS IDWOS:000283959900004
Citation statistics
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/8479
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Yan, Chang-Feng,Cheng, Fei-Fei,Hu, Rong-Rong. Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2010,35(21):11693-11699.
APA Yan, Chang-Feng,Cheng, Fei-Fei,&Hu, Rong-Rong.(2010).Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,35(21),11693-11699.
MLA Yan, Chang-Feng,et al."Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 35.21(2010):11693-11699.
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