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Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts
Yan, Chang-Feng1,2; Cheng, Fei-Fei1,2; Hu, Rong-Rong1
2010-11-01
发表期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
ISSN0360-3199
卷号35期号:21页码:11693-11699
产权排序[Yan, Chang-Feng; Cheng, Fei-Fei; Hu, Rong-Rong] Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China; [Yan, Chang-Feng; Cheng, Fei-Fei] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
通讯作者yancf@ms.giec.ac.cn
摘要A series of composite catalysts Ni/CeO2-ZrO2 were prepared via impregnation method with Ni as the active metal. A laboratory-scale fixed-bed reactor was employed to investigate the catalyst performance during hydrogen production by steam reforming bio-oil aqueous fraction. Effects of water-to-bio-oil ratio (W/B), reaction temperature, and the loaded weight of Ni and Ce on the hydrogen production performance of Nil CeO2-ZrO2 catalysts were examined. The obtained results were compared with commercial nickel-based catalysts (Z417). The best performance of Ni/CeO2-ZrO2 catalyst was observed when the Ni and Ce loaded weight were 12% and 7.5% respectively. At W/B = 4.9, T = 800 degrees C, H-2 yield reaches the highest of 69.7% and H-2 content of 61.8% were obtained. Under the same condition, H-2 yield and H-2 content were higher than commercial nickel-based catalysts (Z417). (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
文章类型Article
其他摘要A series of composite catalysts Ni/CeO2-ZrO2 were prepared via impregnation method with Ni as the active metal. A laboratory-scale fixed-bed reactor was employed to investigate the catalyst performance during hydrogen production by steam reforming bio-oil aqueous fraction. Effects of water-to-bio-oil ratio (W/B), reaction temperature, and the loaded weight of Ni and Ce on the hydrogen production performance of Nil CeO2-ZrO2 catalysts were examined. The obtained results were compared with commercial nickel-based catalysts (Z417). The best performance of Ni/CeO2-ZrO2 catalyst was observed when the Ni and Ce loaded weight were 12% and 7.5% respectively. At W/B = 4.9, T = 800 degrees C, H-2 yield reaches the highest of 69.7% and H-2 content of 61.8% were obtained. Under the same condition, H-2 yield and H-2 content were higher than commercial nickel-based catalysts (Z417). (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
关键词Ni/ceo2-zro2 Hydrogen Bio-oil Steam Reforming
学科领域Chemistry ; Electrochemistry ; Energy & Fuels
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.ijhydene.2010.08.083
研究领域[WOS]Chemistry ; Electrochemistry ; Energy & Fuels
URL查看原文
关键词[WOS]ACETIC-ACID ; FAST-PYROLYSIS ; BIOMASS PYROLYSIS ; NICKEL-CATALYSTS ; METAL-CATALYSTS ; MODEL COMPOUNDS ; BED REACTOR ; TEMPERATURE ; ETHANOL ; GASIFICATION
收录类别SCI
语种英语
项目资助者Natural Science Foundation of China [20806082, 50306026]
WOS类目Chemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS记录号WOS:000283959900004
引用统计
被引频次:61[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/8479
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Yan, Chang-Feng,Cheng, Fei-Fei,Hu, Rong-Rong. Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2010,35(21):11693-11699.
APA Yan, Chang-Feng,Cheng, Fei-Fei,&Hu, Rong-Rong.(2010).Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,35(21),11693-11699.
MLA Yan, Chang-Feng,et al."Hydrogen production from catalytic steam reforming of bio-oil aqueous fraction over Ni/CeO2-ZrO2 catalysts".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 35.21(2010):11693-11699.
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