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Metal-free g-C3N4/melem nanorods hybrids for photocatalytic degradation of methyl orange
Mo, Jiamei; Wang, Nan; Zhang, Shaohong; Chen, Xiaoli; Fu, Juan; Chen, Peili; Liang, Zheng; Su, Qiucheng; Li, Xinjun
2022-07-29
发表期刊RESEARCH ON CHEMICAL INTERMEDIATES
ISSN0922-6168
页码15
通讯作者Su, Qiucheng(suqc@ms.giec.ac.cn) ; Li, Xinjun(lixj@ms.giec.ac.cn)
摘要In this work, g-C3N4/melem nanorods hybrids were synthesized via a rapid cooling process with H2SO4-assisted treatments of bulk g-C3N4. The results show that post treatment of pristine g-C3N4 using concentrated H2SO4 can produce a hybrid crystal structure containing both melem and g-C3N4. The melem nanorods were formed based on H2SO4 exfoliation, regrowth process and nanoplates roll-up mechanism through a rapid cooling process. The g-C3N4/melem nanorods hybrids exhibited efficient degradation of methyl orange and the efficiency was nearly 100% in 80 min, which presented much better than bulk g-C3N4 (giving a degradation efficiency of 67% in 80 min). The enhanced photocatalytic performance of g-C3N4/melem nanorods hybrids mainly originates from the synergistic effect of g-C3N4 and melem, which the g-C3N4/melem hybrids can improving the efficiency of photogenerated charge separation of g-C3N4. This study contributes towards an effective strategy for optimizing the crystalline structure and nanostructure of g-C3N4/melem hybrids to enhanced g-C3N4 photodegradation activity.
关键词Metal-free Melem g-C3N4 Nanostructure Photocatalytic degradation
DOI10.1007/s11164-022-04779-6
关键词[WOS]GRAPHITIC CARBON NITRIDE ; FACILE SYNTHESIS ; WATER ; MELEM ; FABRICATION ; PHOSPHORUS ; NANOTUBES
收录类别SCI
语种英语
资助项目Science and Technology Program of Guangzhou, China[201803030019]
WOS研究方向Chemistry
项目资助者Science and Technology Program of Guangzhou, China
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000832807600001
出版者SPRINGER
引用统计
被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/37008
专题中国科学院广州能源研究所
通讯作者Su, Qiucheng; Li, Xinjun
作者单位Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Mo, Jiamei,Wang, Nan,Zhang, Shaohong,et al. Metal-free g-C3N4/melem nanorods hybrids for photocatalytic degradation of methyl orange[J]. RESEARCH ON CHEMICAL INTERMEDIATES,2022:15.
APA Mo, Jiamei.,Wang, Nan.,Zhang, Shaohong.,Chen, Xiaoli.,Fu, Juan.,...&Li, Xinjun.(2022).Metal-free g-C3N4/melem nanorods hybrids for photocatalytic degradation of methyl orange.RESEARCH ON CHEMICAL INTERMEDIATES,15.
MLA Mo, Jiamei,et al."Metal-free g-C3N4/melem nanorods hybrids for photocatalytic degradation of methyl orange".RESEARCH ON CHEMICAL INTERMEDIATES (2022):15.
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