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Municipal solid wastes pyro-gasification using high-temperature flue gas as heating resource and gasifying agent
Ge, Shaoheng1,2; Chen, Dezhen1,2; Yin, Lijie1,2; Hong, Liu1,2; Zhou, Hongquan1,3; Huang, Zhen4
2022-07-15
发表期刊WASTE MANAGEMENT
ISSN0956-053X
卷号149页码:114-123
通讯作者Chen, Dezhen(chendezhen@tongji.edu.cn)
摘要With the implementation of municipal solid wastes (MSW) source segregation collection policy, the combustible waste components are suitable for pyrolysis treatment to recover value-added energy such as gas or oil. In this research, the volatile compounds from MSW pyrolysis were reformed by the char obtained from the same process and the high-temperature flue gas (HTFG) of 1200 degrees C was supplying as heating resource and gasifying agent in a tailor-made experimental set-up. The final yields and properties of the syngas, char, and oil after reforming were investigated. Experimental studies showed that the composition of HTFG had a significant influence on the products. As the HTFG being CO2 and its flowrate increased from 0 to 4 L/min/(kgMSW), the energy share in the gas first increased from 8.29 to 15.1 MJ/(kgMSW) with a higher heat value (HHV) of 19.9 MJ/Nm3, then it decreased slightly with a further increase in the flowrate. However, as the HTFG was H2O or the model flue gas (consisting of CO2, H2O, O2 and N2), the higher flowrate always increased the energy share and cold gasification efficiency (CGE) in the gas products. Both CO2 and H2O participated the volatiles' reforming reactions and enhanced char gasification; while the volatiles' reforming inhibited char gasification. When the flowrate of the model flue gas increased from 0 to 12.04 L/min/(kgMSW), the oil and char yields decreased and the CGE increased to more than 75%, which was much higher than that from direct air gasification of MSW; moreover, the gas products had much higher HHVs. This research provides a guidance for producing high-quality syngas from the MSW.
关键词MSW pyrolysis Pyro-gasification High-temperature flue gas Heating source CGE
DOI10.1016/j.wasman.2022.06.010
关键词[WOS]STEAM GASIFICATION ; CHAR GASIFICATION ; PYROLYSIS ; TAR ; CO2 ; TECHNOLOGIES ; REACTIVITY ; MECHANISM ; HYDROGEN ; H2O
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[51776141] ; Shanghai Municipal Science and Technology Commission[20230712900]
WOS研究方向Engineering ; Environmental Sciences & Ecology
项目资助者National Natural Science Foundation of China ; Shanghai Municipal Science and Technology Commission
WOS类目Engineering, Environmental ; Environmental Sciences
WOS记录号WOS:000818587800003
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/36962
专题中国科学院广州能源研究所
通讯作者Chen, Dezhen
作者单位1.Tongji Univ, Thermal & Environm Engn Inst, Sch Mech Engn, 1239 Siping Rd, Shanghai 200092, Peoples R China
2.Shanghai Engn Res Ctr Multisource Solid Wastes Cop, 1239 Siping Rd, Shanghai 200092, Peoples R China
3.Shanghai Inst Design & Res Environm Engn Co Ltd Sh, Shanghai 200031, Peoples R China
4.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou, Peoples R China
推荐引用方式
GB/T 7714
Ge, Shaoheng,Chen, Dezhen,Yin, Lijie,et al. Municipal solid wastes pyro-gasification using high-temperature flue gas as heating resource and gasifying agent[J]. WASTE MANAGEMENT,2022,149:114-123.
APA Ge, Shaoheng,Chen, Dezhen,Yin, Lijie,Hong, Liu,Zhou, Hongquan,&Huang, Zhen.(2022).Municipal solid wastes pyro-gasification using high-temperature flue gas as heating resource and gasifying agent.WASTE MANAGEMENT,149,114-123.
MLA Ge, Shaoheng,et al."Municipal solid wastes pyro-gasification using high-temperature flue gas as heating resource and gasifying agent".WASTE MANAGEMENT 149(2022):114-123.
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