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Adsorption performance of tetracycline by the biomass ash derived from the pyrolysis of FeCl3-activated municipal sludge without gas protection
Yu, Chunmu1,2; Chen, Xiaojuan2; Li, Ning2,3; Yao, Liang4; Zhou, Yu5; Lu, Kaihong5; Chen, Jieming4
2022-06-06
发表期刊ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
ISSN0944-1344
页码10
通讯作者Li, Ning(lining@ms.giec.ac.cn)
摘要The municipal sludge activated by FeCl3 solution was pyrolyzed at 500 degrees C without gas protection, and the pyrolysis products, named as biomass ash, could effectively adsorb tetracycline (TC) from aqueous solution. Different FeCl3 concentrations could directly affect the physicochemical properties of the biomass ash, so that the biomass ash as adsorbent showed different adsorption efficiency toward TC. The activation of FeCl3 increased the oxygen-containing functional groups and surface polarities of the biomass ash. When the concentration of FeCl3 solution was 0.5 mol/L, the biomass ash behaved the maximum specific surface area (37.74 m(2)/g) and the best adsorption efficiency. The pseudo-second-order kinetics model and the Freundlich multi-molecule model could fully explain the TC adsorption process by the biomass ash pyrolyzed from municipal sludge activated by FeCl3. Moreover, the adsorption mechanism was mainly attributed to the chemical adsorption.
关键词Municipal sludge Activation Ferric chloride Pyrolysis Tetracycline
DOI10.1007/s11356-022-20533-2
关键词[WOS]SEWAGE-SLUDGE ; BIOCHAR PROPERTIES ; BLACK CARBON ; WASTE-WATER ; REMOVAL ; TEMPERATURE ; ACTIVATION ; MICROWAVE ; ADSORBENT ; PB(II)
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[21908220] ; Doctoral Fund of Ministry of Education of China[2019M663139] ; Doctoral Fund of Ministry of Education of China[2020M672854] ; Natural Science Foundation of Guangdong Province of China[2020A1515010364] ; Natural Science Foundation of Guangzhou[202102020825]
WOS研究方向Environmental Sciences & Ecology
项目资助者National Natural Science Foundation of China ; Doctoral Fund of Ministry of Education of China ; Natural Science Foundation of Guangdong Province of China ; Natural Science Foundation of Guangzhou
WOS类目Environmental Sciences
WOS记录号WOS:000807812000015
出版者SPRINGER HEIDELBERG
引用统计
被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/36742
专题中国科学院广州能源研究所
通讯作者Li, Ning
作者单位1.Xiangtan Univ, Sch Chem Engn, Key Lab Green Catalysis & Chem React Engn Hunan P, Xiangtan 411105, Peoples R China
2.Foshan Univ, Coll Environm & Chem Engn, Foshan 528000, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510650, Peoples R China
4.Foshan Univ, Coll Transportat & Civil Architecture, Foshan 528000, Peoples R China
5.Foshan Univ, Sch Food Sci & Engn, Foshan 528000, Peoples R China
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GB/T 7714
Yu, Chunmu,Chen, Xiaojuan,Li, Ning,et al. Adsorption performance of tetracycline by the biomass ash derived from the pyrolysis of FeCl3-activated municipal sludge without gas protection[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2022:10.
APA Yu, Chunmu.,Chen, Xiaojuan.,Li, Ning.,Yao, Liang.,Zhou, Yu.,...&Chen, Jieming.(2022).Adsorption performance of tetracycline by the biomass ash derived from the pyrolysis of FeCl3-activated municipal sludge without gas protection.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,10.
MLA Yu, Chunmu,et al."Adsorption performance of tetracycline by the biomass ash derived from the pyrolysis of FeCl3-activated municipal sludge without gas protection".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2022):10.
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