Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production

doi:10.1016/j.energy.2022.123342

GIEC OpenIR

	Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production
	Wang, Shuxiao 1,2,5,6; Zhang, Yuyuan 4; Shan, Rui 1,3,5,6; Gu, Jing 1,3,5,6; Yuan, Haoran1,3,5,6 ; Chen, Yong1,2,3,5,6
	2022-05-01
发表期刊	ENERGY
ISSN	0360-5442
卷号	246 页码:9
通讯作者	Yuan, Haoran(yuanhr@ms.giec.ac.cn)
摘要	The removal of biomass tar is the key technology in the pyrolysis and gasification technology, and the advantages of solid waste pyrolysis char in tar removal gradually become prominent. In this paper, the tar model compound (benzene) was catalytic reformed by a novel hybrid carrier catalysts using a laboratory dual-stage reactor. The hybrid carrier catalyst was prepared by wet impregnation method with nickel active substance, and the carrier was a two-material mixture of peat char and sludge char. In the reaction of steam reforming benzene, the effects of temperature (600-800 degrees C) and nickel load (5%-20%) on benzene conversion were investigated, showing that the catalyst have good benzene removal ability (91.8%) and the gas product with high syngas content (93.6%) was obtained. The surface properties of the catalyst was detected by SEM, EDS, BET and XRD detection, in order to prove that the catalytic performance was related to surface nanoparticles and abundant active sites. The novel hybrid carrier catalyst can effectively remove the aromatic tar and produce syngas with high performance. (c) 2022 Elsevier Ltd. All rights reserved.
关键词	Thermochemical Catalytic reforming Syngas Tar removal Hydrogen Pyrolysis char
DOI	10.1016/j.energy.2022.123342
关键词[WOS]	MICROWAVE PYROLYSIS ; BOTTOM ASH ; RICE HUSK ; CRACKING ; GASIFICATION ; TOLUENE ; SLUDGE ; CARBON ; DECOMPOSITION ; CONVERSION
收录类别	SCI
语种	英语
资助项目	National Key R&D Pro-gram of China[2018YFC1901200] ; Key Special Project for Intro-duced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)[GML2019ZD0101] ; National Natural Science Foundation of China[51906248] ; National Natural Science Foundation of China[51906045] ; CAS Key Laboratory of Renewable Energy[E029040101] ; Guangdong Province Science and Technology Planning Project[2019B110210003]
WOS研究方向	Thermodynamics ; Energy & Fuels
项目资助者	National Key R&D Pro-gram of China ; Key Special Project for Intro-duced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) ; National Natural Science Foundation of China ; CAS Key Laboratory of Renewable Energy ; Guangdong Province Science and Technology Planning Project
WOS类目	Thermodynamics ; Energy & Fuels
WOS记录号	WOS:000791830300004
出版者	PERGAMON-ELSEVIER SCIENCE LTD
引用统计	被引频次：7[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/36380
专题	中国科学院广州能源研究所
通讯作者	Yuan, Haoran
作者单位	1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.Nanjing Tech Univ, Nanjing 211816, Peoples R China 3.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China 4.Foshan Univ, Sch Mat Sci & Hydrogen Energy, Foshan, Peoples R China 5.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 6.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
第一作者单位	中国科学院广州能源研究所
推荐引用方式 GB/T 7714	Wang, Shuxiao,Zhang, Yuyuan,Shan, Rui,et al. Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production[J]. ENERGY,2022,246:9.
APA	Wang, Shuxiao,Zhang, Yuyuan,Shan, Rui,Gu, Jing,Yuan, Haoran,&Chen, Yong.(2022).Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production.ENERGY,246,9.
MLA	Wang, Shuxiao,et al."Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production".ENERGY 246(2022):9.