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Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production
Wang, Shuxiao1,2,5,6; Zhang, Yuyuan4; Shan, Rui1,3,5,6; Gu, Jing1,3,5,6; Yuan, Haoran1,3,5,6; Chen, Yong1,2,3,5,6
2022-05-01
Source PublicationENERGY
ISSN0360-5442
Volume246Pages:9
Corresponding AuthorYuan, Haoran(yuanhr@ms.giec.ac.cn)
AbstractThe removal of biomass tar is the key technology in the pyrolysis and gasification technology, and the advantages of solid waste pyrolysis char in tar removal gradually become prominent. In this paper, the tar model compound (benzene) was catalytic reformed by a novel hybrid carrier catalysts using a laboratory dual-stage reactor. The hybrid carrier catalyst was prepared by wet impregnation method with nickel active substance, and the carrier was a two-material mixture of peat char and sludge char. In the reaction of steam reforming benzene, the effects of temperature (600-800 degrees C) and nickel load (5%-20%) on benzene conversion were investigated, showing that the catalyst have good benzene removal ability (91.8%) and the gas product with high syngas content (93.6%) was obtained. The surface properties of the catalyst was detected by SEM, EDS, BET and XRD detection, in order to prove that the catalytic performance was related to surface nanoparticles and abundant active sites. The novel hybrid carrier catalyst can effectively remove the aromatic tar and produce syngas with high performance. (c) 2022 Elsevier Ltd. All rights reserved.
KeywordThermochemical Catalytic reforming Syngas Tar removal Hydrogen Pyrolysis char
DOI10.1016/j.energy.2022.123342
WOS KeywordMICROWAVE PYROLYSIS ; BOTTOM ASH ; RICE HUSK ; CRACKING ; GASIFICATION ; TOLUENE ; SLUDGE ; CARBON ; DECOMPOSITION ; CONVERSION
Indexed BySCI
Language英语
Funding ProjectNational Key R&D Pro-gram of China[2018YFC1901200] ; Key Special Project for Intro-duced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)[GML2019ZD0101] ; National Natural Science Foundation of China[51906248] ; National Natural Science Foundation of China[51906045] ; CAS Key Laboratory of Renewable Energy[E029040101] ; Guangdong Province Science and Technology Planning Project[2019B110210003]
WOS Research AreaThermodynamics ; Energy & Fuels
Funding OrganizationNational Key R&D Pro-gram of China ; Key Special Project for Intro-duced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) ; National Natural Science Foundation of China ; CAS Key Laboratory of Renewable Energy ; Guangdong Province Science and Technology Planning Project
WOS SubjectThermodynamics ; Energy & Fuels
WOS IDWOS:000791830300004
PublisherPERGAMON-ELSEVIER SCIENCE LTD
Citation statistics
Cited Times:8[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/36380
Collection中国科学院广州能源研究所
Corresponding AuthorYuan, Haoran
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Nanjing Tech Univ, Nanjing 211816, Peoples R China
3.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China
4.Foshan Univ, Sch Mat Sci & Hydrogen Energy, Foshan, Peoples R China
5.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
6.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Wang, Shuxiao,Zhang, Yuyuan,Shan, Rui,et al. Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production[J]. ENERGY,2022,246:9.
APA Wang, Shuxiao,Zhang, Yuyuan,Shan, Rui,Gu, Jing,Yuan, Haoran,&Chen, Yong.(2022).Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production.ENERGY,246,9.
MLA Wang, Shuxiao,et al."Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production".ENERGY 246(2022):9.
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