Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support

doi:10.1039/d1nj06013a

GIEC OpenIR

	Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support
	Luo, Fengying 1,2; Wang, Zeyu 1,2; Li, Xiangnan 1; Lang, Lin1 ; Li, Xinjun1 ; Yin, Xiuli1
	2022-05-16
Source Publication	NEW JOURNAL OF CHEMISTRY
ISSN	1144-0546
Volume	46 Issue:19 Pages:9304-9311
Corresponding Author	Li, Xinjun() ; Yin, Xiuli()
Abstract	Highly dispersed Ni-based catalysts were derived from self-reconstruction of the LaNiO3 perovskite, which were prepared via the sol-gel process. Activity measurements indicated that the as-prepared catalysts exhibit an excellent dry methane reforming catalytic performance, which can achieve CH4 conversion of 84.17% and 83.35% at 650 degrees C at a gas hourly space velocity (GHSV) of 128 L (g(cat) h)(-1). The physicochemical characterization of the as-prepared catalysts suggested that the transition layer of La2NiO4 is formed between metallic Ni-0 and the La(OH)(3) support. The Ni-0-Ni2+ dipole on the support is relevant to the catalytic activity for the dry methane reforming reaction.
DOI	10.1039/d1nj06013a
WOS Keyword	RAY PHOTOELECTRON-SPECTROSCOPY ; SYNGAS PRODUCTION ; OXIDE CATALYSTS ; CARBON-DIOXIDE ; PERFORMANCE ; CH4 ; REDUCTION ; NI/LA2O3
Indexed By	SCI
Language	英语
Funding Project	National Key R&D Program of China[2019YFB1503902] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA21060600] ; Science and Technology Program of Guangzhou[202002030126]
WOS Research Area	Chemistry
Funding Organization	National Key R&D Program of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Science and Technology Program of Guangzhou
WOS Subject	Chemistry, Multidisciplinary
WOS ID	WOS:000788237400001
Publisher	ROYAL SOC CHEMISTRY
Citation statistics	Cited Times:4[WOS] [WOS Record] [Related Records in WOS]
Document Type	期刊论文
Identifier	http://ir.giec.ac.cn/handle/344007/36298
Collection	中国科学院广州能源研究所
Corresponding Author	Li, Xinjun; Yin, Xiuli
Affiliation	1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
First Author Affilication	GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation GB/T 7714	Luo, Fengying,Wang, Zeyu,Li, Xiangnan,et al. Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support[J]. NEW JOURNAL OF CHEMISTRY,2022,46(19):9304-9311.
APA	Luo, Fengying,Wang, Zeyu,Li, Xiangnan,Lang, Lin,Li, Xinjun,&Yin, Xiuli.(2022).Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support.NEW JOURNAL OF CHEMISTRY,46(19),9304-9311.
MLA	Luo, Fengying,et al."Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support".NEW JOURNAL OF CHEMISTRY 46.19(2022):9304-9311.

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