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Investigation of the formation characteristics of methane hydrate in frozen porous media
Zhang, Xuemin1,2,3; Zhang, Shanling1,2; Li, Yinhui1,2; Li, Jinping1,2,3; Wang, Yingmei1,2,4; Yang, Li1,2
2022-02-01
Source PublicationPETROLEUM SCIENCE AND TECHNOLOGY
ISSN1091-6466
Pages18
Corresponding AuthorZhang, Xuemin(zxm2010lut@163.com)
AbstractThe replacement technique of CO2-CH4 hydrate in naturally occurring gas hydrates is a promising method for achieving CO2 storage and CH4 recovery in permafrost regions. Revealing the formation characteristics of CH4 hydrate becomes an urgent need in porous medium below the freezing point. For this purpose, the formation experiment was carried out under different conditions and the formation characteristics were systematically investigated. The result indicated that the initial pressure was the key factor affecting the formation process of CH4 hydrate. And the final pressure drop was greater at higher initial pressure conditions. The final pressure drop reached to 0.92 MPa when the initial pressure was 9 MPa under the same temperature conditions. The results also illustrated that, the formation rate of hydrate was the fastest when the temperatures were closely to the freezing point. The average formation rate of CH4 hydrate reached to 0.646 mmol/h when the temperature was 273.15 K. Moreover, the smaller the particle size was, the higher the final conversion rate of ice. The final conversion rate reached to 56.5% when the initial pressure was 9 MPa. The results are of significance for exploiting natural gas hydrate in the permafrost regions.
KeywordCH4 hydrate conversion rate formation rate freezing point porous media
DOI10.1080/10916466.2022.2036191
WOS KeywordGAS HYDRATE ; WATER ; DISSOCIATION ; STORAGE ; SEDIMENTS ; EQUILIBRIUM ; PRESSURE ; HUFF ; ICE
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51906093] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[E029kf1501] ; Hongliu Excellent Young Talents Support Program of Lanzhou University of Technology (2018)
WOS Research AreaEnergy & Fuels ; Engineering
Funding OrganizationNational Natural Science Foundation of China ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences ; Hongliu Excellent Young Talents Support Program of Lanzhou University of Technology (2018)
WOS SubjectEnergy & Fuels ; Engineering, Chemical ; Engineering, Petroleum
WOS IDWOS:000760096400001
PublisherTAYLOR & FRANCIS INC
Citation statistics
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/35873
Collection中国科学院广州能源研究所
Corresponding AuthorZhang, Xuemin
Affiliation1.Lanzhou Univ Technol, Coll Energy & Power Engn, Lanzhou, Peoples R China
2.Gansu Prov Key Lab Complementary Energy Syst Biom, Lanzhou, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou, Peoples R China
4.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Frozen Soil Engn, Lanzhou, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Zhang, Xuemin,Zhang, Shanling,Li, Yinhui,et al. Investigation of the formation characteristics of methane hydrate in frozen porous media[J]. PETROLEUM SCIENCE AND TECHNOLOGY,2022:18.
APA Zhang, Xuemin,Zhang, Shanling,Li, Yinhui,Li, Jinping,Wang, Yingmei,&Yang, Li.(2022).Investigation of the formation characteristics of methane hydrate in frozen porous media.PETROLEUM SCIENCE AND TECHNOLOGY,18.
MLA Zhang, Xuemin,et al."Investigation of the formation characteristics of methane hydrate in frozen porous media".PETROLEUM SCIENCE AND TECHNOLOGY (2022):18.
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