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Metal-free photocatalyst of few-layer phosphorene with excellent activity under different light conditions
Yao, Liang1; Chen, Xiaojuan1; Yu, Chunmu1; Chen, Jieming1; Lai, Yiqi1; Li, Ning2
2022
发表期刊MATERIALS LETTERS
ISSN0167-577X
卷号306页码:4
通讯作者Chen, Xiaojuan(xjchen0218@163.com) ; Li, Ning(lining@ms.giec.ac.cn)
摘要Herein, liquid exfoliation method was employed to prepare metal-free photocatalyst of few-layer phosphorene using black phosphorus as the precursor and its physicochemical properties were systematically characterized. The photocatalytic degradation experiments show that phosphorene exhibits more excellent photocatalytic activity toward tetracycline (TC) degradation under UV light irradiation with deoxidation. Moreover, the photodegradation rate constant of TC during the first 15 min of reaction is 0.2004 min(-1), which is 4.61 times of that under the pure UV light irradiation. Furthermore, the catalytic mechanism of phosphorene toward TC degradation was proposed and the excellent photocatalytic performance is mainly contributed to the efficient separation of photogenerated h(+) and e(-).
关键词Semiconductors Phosphorene Photocatalysis Deoxidation
DOI10.1016/j.matlet.2021.130884
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[51708116] ; National Natural Science Foundation of China[21908220] ; Doctoral Fund of Ministry of Education of China[2019M663139] ; Doctoral Fund of Ministry of Education of China[2020M672854] ; Natural Science Foundation of Guangdong Province of China[2020A1515010364]
WOS研究方向Materials Science ; Physics
项目资助者National Natural Science Foundation of China ; Doctoral Fund of Ministry of Education of China ; Natural Science Foundation of Guangdong Province of China
WOS类目Materials Science, Multidisciplinary ; Physics, Applied
WOS记录号WOS:000705842100010
出版者ELSEVIER
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/35039
专题中国科学院广州能源研究所
通讯作者Chen, Xiaojuan; Li, Ning
作者单位1.Foshan Univ, Foshan 528000, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510650, Peoples R China
推荐引用方式
GB/T 7714
Yao, Liang,Chen, Xiaojuan,Yu, Chunmu,et al. Metal-free photocatalyst of few-layer phosphorene with excellent activity under different light conditions[J]. MATERIALS LETTERS,2022,306:4.
APA Yao, Liang,Chen, Xiaojuan,Yu, Chunmu,Chen, Jieming,Lai, Yiqi,&Li, Ning.(2022).Metal-free photocatalyst of few-layer phosphorene with excellent activity under different light conditions.MATERIALS LETTERS,306,4.
MLA Yao, Liang,et al."Metal-free photocatalyst of few-layer phosphorene with excellent activity under different light conditions".MATERIALS LETTERS 306(2022):4.
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