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Novel visible-light-driven SrCoO3/Ag3PO4 heterojunction with enhanced photocatalytic performance for tetracycline degradation
Li, Ning1; Chen, Jieming2; Chen, Xiaojuan2,3; Lai, Yiqi2; Yu, Chunmu3; Yao, Liang2; Liang, Yunqing3
2021-09-09
发表期刊ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
ISSN0944-1344
页码14
通讯作者Chen, Xiaojuan(xjchen0218@163.com)
摘要The semiconductor photocatalytic technology has been considerably studied due to its excellent catalytic performance in water pollution control. Herein, in this study, novel SrCoO3/Ag3PO4 composite materials with different SrCoO3 content were synthesized via a simple hydrothermal synthesis method. The characteristics of the as-prepared samples were detected through SEM/HRTEM, XRD, UV-vis DRS, PL, ESR, FT-IR, and XPS techniques, and then, the photocatalytic performance of SrCoO3/Ag3PO4 toward the degradation of tetracycline was investigated. When the mass ratio of SrCoO3 and Ag3PO4 in the composite was 1:1.5, the degradation rate constant of tetracycline in SrCoO3/Ag3PO4 (1:1.5) system is 0.0102 min(-1), which is 1.7 times that of the Ag3PO4, and 3.78 times that of the SrCoO3. In addition, reactive species were also analyzed through the free radical trapping experiment and DMPO spin-trapping ESR spectra analysis, showing that OH center dot, h(+), and O(2)(center dot-)participated in the catalytic degradation process of tetracycline to varying degrees. Finally, the photocatalytic mechanism of SrCoO3/Ag3PO4 was also proposed.
关键词SrCoO3 Ag3PO4 Semiconductors Visible light Photocatalytic mechanism Tetracycline
DOI10.1007/s11356-021-16338-4
关键词[WOS]HIGHLY EFFICIENT ; COMPOSITE ; HYDROCHLORIDE ; AG3PO4 ; FILM
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[51708116] ; National Natural Science Foundation of China[21908220] ; Doctoral Fund of Ministry of Education of China[2019M663139] ; Doctoral Fund of Ministry of Education of China[2020M672854] ; Natural Science Foundation of Guangdong Province of China[2020A1515010364] ; 13th Five-Year Plan of Educational Science in Guangdong Province special Innovation Projects (Natural Science)[2018KTSCX243] ; Scientific Research Foundation for High-level Talents of Foshan University[gg07014]
WOS研究方向Environmental Sciences & Ecology
项目资助者National Natural Science Foundation of China ; Doctoral Fund of Ministry of Education of China ; Natural Science Foundation of Guangdong Province of China ; 13th Five-Year Plan of Educational Science in Guangdong Province special Innovation Projects (Natural Science) ; Scientific Research Foundation for High-level Talents of Foshan University
WOS类目Environmental Sciences
WOS记录号WOS:000694622200020
出版者SPRINGER HEIDELBERG
引用统计
被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/33852
专题中国科学院广州能源研究所
通讯作者Chen, Xiaojuan
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510650, Peoples R China
2.Foshan Univ, Sch Transportat Civil Engn & Architecture, Foshan 528225, Peoples R China
3.Foshan Univ, Sch Environm & Chem Engn, Foshan 528000, Peoples R China
第一作者单位中国科学院广州能源研究所
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GB/T 7714
Li, Ning,Chen, Jieming,Chen, Xiaojuan,et al. Novel visible-light-driven SrCoO3/Ag3PO4 heterojunction with enhanced photocatalytic performance for tetracycline degradation[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2021:14.
APA Li, Ning.,Chen, Jieming.,Chen, Xiaojuan.,Lai, Yiqi.,Yu, Chunmu.,...&Liang, Yunqing.(2021).Novel visible-light-driven SrCoO3/Ag3PO4 heterojunction with enhanced photocatalytic performance for tetracycline degradation.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,14.
MLA Li, Ning,et al."Novel visible-light-driven SrCoO3/Ag3PO4 heterojunction with enhanced photocatalytic performance for tetracycline degradation".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2021):14.
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