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Catalytic fast pyrolysis of waste mixed cloth for the production of value-added chemicals
Zhang, Jun; Gu, Jing; Yuan, Haoran1; Chen, Yong
2021-05-15
发表期刊WASTE MANAGEMENT
ISSN0956-053X
卷号127页码:141-146
通讯作者Yuan, Haoran(yuanhr@ms.giec.ac.cn)
摘要In the present study, catalytic fast pyrolysis of waste mixed cloth in an ex-situ method using hierarchical HZSM and commercial CaO was investigated. Pyrolysis of waste mixed cloth in a temperature range of 450 degrees C to 750 degrees C mainly allowed for the formation of levoglucosan without any catalysts. The utilization of HZSM with Br & oslash;nsted/Lewis acid sites on micro-and mesoporous structures significantly contributed to monocyclic/dicyclic chemicals production, mainly referring to monoaromatics and naphthalene-based derivatives, especially in the case of high heating rates and catalyst usages. Furthermore, CaO revealed strong deoxygenation performance for the transformation of waste mixed cloth into low oxygen-containing chemicals, such as ketones, aliphatic hydrocarbons and aromatics. The present research thus highlights a feasible route for the catalytic upgrading of waste mixed cloth into some kinds of value-added chemicals. (c) 2021 Elsevier Ltd. All rights reserved.
关键词Catalytic fast pyrolysis Waste mixed cloth Levoglucosan Aromatics
DOI10.1016/j.wasman.2021.04.036
关键词[WOS]BIO-OIL ; HIERARCHICAL ZSM-5 ; CO-PYROLYSIS ; BIOMASS ; CELLULOSE ; DEOXYGENATION ; ZEOLITES ; QUALITY ; CAO
收录类别SCI
语种英语
资助项目National Key R&D Program of China[2018YFC1901200] ; National Natural Science Foundation of China[51976222] ; National Natural Science Foundation of China[51976223] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)[GML2019ZD0101] ; Natural Science Foundation of Guangdong Province, China[2018A030313856] ; Open Project of State Key Laboratory of Clean Energy Utilization, Zhejiang University[ZJUCEU2020023] ; Science and Technology Planning Project of Guangzhou[201904010351]
WOS研究方向Engineering ; Environmental Sciences & Ecology
项目资助者National Key R&D Program of China ; National Natural Science Foundation of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) ; Natural Science Foundation of Guangdong Province, China ; Open Project of State Key Laboratory of Clean Energy Utilization, Zhejiang University ; Science and Technology Planning Project of Guangzhou
WOS类目Engineering, Environmental ; Environmental Sciences
WOS记录号WOS:000656420800015
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/33320
专题中国科学院广州能源研究所
通讯作者Yuan, Haoran
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China
3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
4.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Jun,Gu, Jing,Yuan, Haoran,et al. Catalytic fast pyrolysis of waste mixed cloth for the production of value-added chemicals[J]. WASTE MANAGEMENT,2021,127:141-146.
APA Zhang, Jun,Gu, Jing,Yuan, Haoran,&Chen, Yong.(2021).Catalytic fast pyrolysis of waste mixed cloth for the production of value-added chemicals.WASTE MANAGEMENT,127,141-146.
MLA Zhang, Jun,et al."Catalytic fast pyrolysis of waste mixed cloth for the production of value-added chemicals".WASTE MANAGEMENT 127(2021):141-146.
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