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Effects of gas occurrence pattern on distribution and morphology characteristics of gas hydrates in porous media
Kou, Xuan1,2,3,4,5; Li, Xiao-Sen1,2,3,4; Wang, Yi1,2,3,4; Liu, Jian-Wu1,2,3,4; Chen, Zhao-Yang1,2,3,4
2021-07-01
发表期刊ENERGY
ISSN0360-5442
卷号226页码:12
通讯作者Li, Xiao-Sen(lixs@ms.giec.ac.cn) ; Wang, Yi(wangyi@ms.giec.ac.cn)
摘要Natural gas hydrates have attracted much attention in recent years. It is important to investigate the effects of gas occurrence pattern on hydrate growth habits since distribution and morphology characteristics of gas hydrates have significant effects on physical properties of hydrate-bearing reservoirs. In this work, the differences in distribution and morphology properties of gas hydrates under two gas occurrence patterns have been analyzed via the X-ray computed tomography for the first time. Experimental results reveal direct correlations between the hydrate growth habit and the gas occurrence pattern. In the presence of free gas, grain-attaching hydrates are formed at the arc-shaped contact surface of gas and water, and mass transfer at the gas-water interface is the key controlling factor in hydrate formation process. In the presence of dissolved gas, dispersed and dendritic hydrates are formed in liquid phase as the result of gas solubility change, and gas diffusion is the crucial factor that influences the growth habit and morphology of gas hydrates during hydrate formation from dissolved gas. Besides, the maximum saturation of dendritic hydrates formed from dissolved gas is limited by the gas solubility. These conclusions are valuable in the improvement of prediction accuracy of gas production from hydrate-bearing sediments. (c) 2021 Elsevier Ltd. All rights reserved.
关键词Gas hydrates Morphology characteristics Distribution Dissolved gas X-ray CT
DOI10.1016/j.energy.2021.120401
关键词[WOS]METHANE-HYDRATE ; BEARING SEDIMENTS ; THERMAL-STIMULATION ; DISSOLVED METHANE ; PORE HABIT ; WATER ; PERMEABILITY ; DISSOCIATION ; GROWTH ; DEPRESSURIZATION
收录类别SCI
语种英语
资助项目Key Program of National Natural Science Foundation of China[51736009] ; National Natural Science Foundation of China[51676190] ; Guangdong Special Support Program-Local innovation and entrepreneurship team project[2019BT02L278] ; Special Project for Marine Economy Development of Guangdong Province[GDME-2018D002] ; Special Project for Marine Economy Development of Guangdong Province[GDME-2020D044] ; Youth Innovation Promotion Association CAS[2018382] ; Science and Technology Apparatus Development Program of the Chinese Academy of Sciences[YJKYYQ20200061] ; Fundamental Research & Applied Fundamental Research Major Project of Guangdong Province[2019B030302004] ; Fundamental Research & Applied Fundamental Research Major Project of Guangdong Province[2020B0301030003]
WOS研究方向Thermodynamics ; Energy & Fuels
项目资助者Key Program of National Natural Science Foundation of China ; National Natural Science Foundation of China ; Guangdong Special Support Program-Local innovation and entrepreneurship team project ; Special Project for Marine Economy Development of Guangdong Province ; Youth Innovation Promotion Association CAS ; Science and Technology Apparatus Development Program of the Chinese Academy of Sciences ; Fundamental Research & Applied Fundamental Research Major Project of Guangdong Province
WOS类目Thermodynamics ; Energy & Fuels
WOS记录号WOS:000649666000013
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:30[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/33123
专题中国科学院广州能源研究所
通讯作者Li, Xiao-Sen; Wang, Yi
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.CAS Key Lab Gas Hydrate, Guangzhou 510640, Peoples R China
3.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
4.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Peoples R China
5.Univ Chinese Acad Sci, Beijing 100083, Peoples R China
第一作者单位中国科学院广州能源研究所
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Kou, Xuan,Li, Xiao-Sen,Wang, Yi,et al. Effects of gas occurrence pattern on distribution and morphology characteristics of gas hydrates in porous media[J]. ENERGY,2021,226:12.
APA Kou, Xuan,Li, Xiao-Sen,Wang, Yi,Liu, Jian-Wu,&Chen, Zhao-Yang.(2021).Effects of gas occurrence pattern on distribution and morphology characteristics of gas hydrates in porous media.ENERGY,226,12.
MLA Kou, Xuan,et al."Effects of gas occurrence pattern on distribution and morphology characteristics of gas hydrates in porous media".ENERGY 226(2021):12.
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