Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media

doi:10.1080/15435075.2021.1875473

GIEC OpenIR

	Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media
	Zhang, Xuemin 1,2,3; Li, Jinping 1,2; Wang, Jiaxian 1,2; Wu, Qingbai 1,4; Wang, Yingmei 1,2; Yao, Ze 1,2
	2021-01-22
发表期刊	INTERNATIONAL JOURNAL OF GREEN ENERGY
ISSN	1543-5075
页码	10
通讯作者	Zhang, Xuemin(zxm2010lut@163.com)
摘要	Gas hydrate-based technology is a promising method for solidifying and sequestrating of CO2 gas into stratum sediments to reduce anthropogenic CO2 emissions and realize the exploitation of natural gas hydrate in the permafrost regions. In order to clarify the formation characteristics of CO2 hydrate in the porous media under condition of below the freezing point, the experiments were conducted in the frozen quartz sands. And the formation rate, the conversion rate and the gas storage capacities for CO2 hydrate were investigated through experimental study in the porous media. The results showed that, under the same temperature and initial pressure conditions, the formation rate, the conversion rate, and the gas storage capacities of hydrate increased with the decrease of particle sizes of the frozen quartz sands. And the ice content of the frozen quartz sands played little influence on the formation rate and the conversion rate of hydrate at the same particle size. Furthermore, the average formation rate attained 0.000544 mol center dot h(-1) in porous media below the freezing point. The conversion rate of ice attained 70.14, 81.72, and 90.61% in the frozen quartz sands with particle sizes of 500, 380, and 250 mu m, respectively. The results also illustrated that, the gas-storage capacity of hydrate achieved 127.58, 144.04, and 152.65 L/L in the corresponding porous media. These results are of signi?cance for guiding capture and sequestration of CO2 gas in the form of gas hydrate in stratum sediments.
关键词	Gas hydrate porous media CO2 sequestration formation characteristics freezing point
DOI	10.1080/15435075.2021.1875473
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51906093] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[Y907ke1001] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[E029kf1501]
WOS研究方向	Thermodynamics ; Science & Technology - Other Topics ; Energy & Fuels
项目资助者	National Natural Science Foundation of China ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences
WOS类目	Thermodynamics ; Green & Sustainable Science & Technology ; Energy & Fuels
WOS记录号	WOS:000619743900001
出版者	TAYLOR & FRANCIS INC
引用统计	被引频次：5[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/32687
专题	中国科学院广州能源研究所
通讯作者	Zhang, Xuemin
作者单位	1.Lanzhou Univ Technol, Western China Res Ctr Energy & Environm, Lanzhou, Peoples R China 2.Key Lab Complementary Energy Syst Biomass & Solar, Lanzhou, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou, Peoples R China 4.Chinese Acad Sci, Cold & Arid Reg Environm & Engn Res Inst, State Key Lab Frozen Soil Engn, Lanzhou, Peoples R China
第一作者单位	中国科学院广州能源研究所
推荐引用方式 GB/T 7714	Zhang, Xuemin,Li, Jinping,Wang, Jiaxian,et al. Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media[J]. INTERNATIONAL JOURNAL OF GREEN ENERGY,2021:10.
APA	Zhang, Xuemin,Li, Jinping,Wang, Jiaxian,Wu, Qingbai,Wang, Yingmei,&Yao, Ze.(2021).Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media.INTERNATIONAL JOURNAL OF GREEN ENERGY,10.
MLA	Zhang, Xuemin,et al."Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media".INTERNATIONAL JOURNAL OF GREEN ENERGY (2021):10.