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Aqueous Cr(VI) removal by biochar derived from waste mangosteen shells: Role of pyrolysis and modification on its absorption process
Shan, Rui1,2,3,4; Shi, Yueyue1,2,3; Gu, Jing1,2,3,4; Bi, Jingwang1,2,3,4; Yuan, Haoran1,2,3,4; Luo, Bo5; Chen, Yong1,2,3,4
2020-08-01
发表期刊JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
卷号8期号:4页码:10
通讯作者Yuan, Haoran(yuanhr@ms.giec.ac.cn)
摘要A series of mangosteen-derived biochars were produced by several modifiers (HCl, KOH and ZnCl2), in different preparation conditions (i.e. pyrolysis temperature, pyrolysis process and impregnation ratio). It indicated that the Z2PT350-700 presented excellent ability for Cr(VI) removal. The physical/chemical properties of the prepared biochar are reflected by the electrostatic interaction, surface complexation, ion exchange occupied primary position in the process of adsorbing Cr(VI). Besides, the effects of reaction time, pH, adsorbent dosage and initial adsorbate concentration on Cr(VI) removal were evaluated. The sorption process of Cr(VI) could be described by the pseudo-second order (PSO) kinetic model and Sips isotherm model. In optimal reaction condition, the surface of Zn2MB350-700 was composed of homogeneous and heterogeneous adsorption and the chemical adsorption dominated in the adsorption process. Therefore, the results suggested that Zn2MB350-700 could be used as an inexpensive and highly efficient adsorbent for Cr removal from water environment.
关键词Modified Mangosteen shell Biochar Cr(VI) Adsorption Pyrolysis
DOI10.1016/j.jece.2020.103885
关键词[WOS]HEXAVALENT CHROMIUM REMOVAL ; HEAVY-METALS ; ACTIVATED CARBONS ; CHROMATE REMOVAL ; POROUS CARBON ; PEEL WASTE ; ADSORPTION ; WATER ; CONTAMINANTS ; TEMPERATURE
收录类别SCI
语种英语
资助项目State's Key Project of Research and Development Plan, China[y804091001] ; National Natural Science Funds of China[51776211] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), China[GML2019ZD0101]
WOS研究方向Engineering
项目资助者State's Key Project of Research and Development Plan, China ; National Natural Science Funds of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), China
WOS类目Engineering, Environmental ; Engineering, Chemical
WOS记录号WOS:000563930800013
出版者ELSEVIER SCI LTD
引用统计
被引频次:44[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/27628
专题中国科学院广州能源研究所
通讯作者Yuan, Haoran
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China
3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
4.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
5.Chongqing Environm & Sanitat Grp Co Ltd, Chongqing 401121, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Shan, Rui,Shi, Yueyue,Gu, Jing,et al. Aqueous Cr(VI) removal by biochar derived from waste mangosteen shells: Role of pyrolysis and modification on its absorption process[J]. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING,2020,8(4):10.
APA Shan, Rui.,Shi, Yueyue.,Gu, Jing.,Bi, Jingwang.,Yuan, Haoran.,...&Chen, Yong.(2020).Aqueous Cr(VI) removal by biochar derived from waste mangosteen shells: Role of pyrolysis and modification on its absorption process.JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING,8(4),10.
MLA Shan, Rui,et al."Aqueous Cr(VI) removal by biochar derived from waste mangosteen shells: Role of pyrolysis and modification on its absorption process".JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 8.4(2020):10.
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