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Calcium-Loaded Municipal Sludge-Biochar as an Efficient and Stable Catalyst for Biodiesel Production from Vegetable Oil
Wang, Yazhuo1,2,3,5; Li, Denian1,2; Zhao, Dandan1,2; Fan, Yukun1,2,3; Bi, Jingwang1,2; Shan, Rui1,2; Yang, Jizhang1,2; Luo, Bo6; Yuan, Haoran1,2,3,4; Ling, Xiang5; Huhe, Taoli6; Chen, Yong1,2,3,4,5
2020-07-21
发表期刊ACS OMEGA
ISSN2470-1343
卷号5期号:28页码:17471-17478
通讯作者Yuan, Haoran(yuanhr@ms.giec.ac.cn)
摘要In this contribution, biochar from municipal sludge was used as a novel matrix for the synthesis of a series of calcium-based heterogeneous catalysts toward biodiesel production. Their catalytic activity was investigated in terms of catalyst loading and calcination temperature during preparation, in addition to the transesterification parameters including the methanol/oil molar ratio, reaction time, and catalyst amount. The highest biodiesel yield up to 93.77% was achieved with the 30Ca/A-SBC-700, and it maintained as high as 84.9% even after 10 cycles of a consecutively alternating catalysis and regeneration process. It was revealed that the porous municipal sludge biochar and autologous SiO2 were accountable for the superior stability of the present catalyst. This work may provide a new path to value-added valorization of sludge waste and also a renewable and efficient catalyst for biodiesel production at a low cost.
DOI10.1021/acsomega.0c01970
关键词[WOS]PALM OIL ; SUPPORTED K2CO3 ; FLY-ASH ; TRANSESTERIFICATION ; CARBON ; SHELL ; TECHNOLOGIES ; METHANOL ; STATE ; OXIDE
收录类别SCI
语种英语
资助项目National Key R&D Program of China[2018YFC1901200] ; National Natural Sciences Foundation of China[51806226] ; Provincial Natural Science Foundation of Guangdong[2017A030310014] ; Provincial Natural Science Foundation of Guangdong[2019A1515011570] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)[GML2019ZD0101]
WOS研究方向Chemistry
项目资助者National Key R&D Program of China ; National Natural Sciences Foundation of China ; Provincial Natural Science Foundation of Guangdong ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000554991800049
出版者AMER CHEMICAL SOC
引用统计
被引频次:14[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/27530
专题中国科学院广州能源研究所
通讯作者Yuan, Haoran
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
2.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China
3.Guangdong Univ Technol, Sch Mat & Energy, Guangzhou 510006, Peoples R China
4.Changzhou Univ, Inst Urban & Rural Min, Sch Petrochem Engn, Changzhou 213164, Peoples R China
5.Nanjing Technol Univ, Sch Mech & Power Engn, Nanjing 211816, Peoples R China
6.Chongqing Environm & Sanitat Grp Co Ltd, Chongqing 401120, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Wang, Yazhuo,Li, Denian,Zhao, Dandan,et al. Calcium-Loaded Municipal Sludge-Biochar as an Efficient and Stable Catalyst for Biodiesel Production from Vegetable Oil[J]. ACS OMEGA,2020,5(28):17471-17478.
APA Wang, Yazhuo.,Li, Denian.,Zhao, Dandan.,Fan, Yukun.,Bi, Jingwang.,...&Chen, Yong.(2020).Calcium-Loaded Municipal Sludge-Biochar as an Efficient and Stable Catalyst for Biodiesel Production from Vegetable Oil.ACS OMEGA,5(28),17471-17478.
MLA Wang, Yazhuo,et al."Calcium-Loaded Municipal Sludge-Biochar as an Efficient and Stable Catalyst for Biodiesel Production from Vegetable Oil".ACS OMEGA 5.28(2020):17471-17478.
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