Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions | |
Shan, Rui1,2,3,4; Lu, Lili1,2,3; Gu, Jing1,2,3,4; Zhang, Yuyuan5; Yuan, Haoran1,2,3,4; Chen, Yong1,2,3,4; Luo, Bo6 | |
2020-08-01 | |
发表期刊 | MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING |
ISSN | 1369-8001 |
卷号 | 114页码:12 |
通讯作者 | Yuan, Haoran(yuanhr@ms.giec.ac.cn) |
摘要 | One set of biochar-coupled Ag and TiO2 composites were successfully fabricated by mixing, calcination, and photodeposition method to remove methyl orange (MO). It was found that all catalysts modified with Ag showed better photocatalytic degradation performance (the highest decolorization efficiency and mineralization efficiency were 97.48% and 85.38%, respectively) than single TiO2 because of the synergy of Ag, TiO2 and biochar. Characterization results indicated that Ag as well as TiO2 acted as electron donor and biochar acted as electron acceptor, which could effectively promote the separation of photogenerated electron hole pairs. In addition, the catalyst exhibited high stability up to 5 cycles and the loss of activity was negligible. And the catalytic degradation process was consistent with the pseudo-first-order kinetic (PFOK) model with the degradation rate constant of 6.29 x 10(2) min(-1). |
关键词 | Ag Surface plasmon resonance Photocatalytic degradation Methyl orange TiO2 |
DOI | 10.1016/j.mssp.2020.105088 |
关键词[WOS] | VISIBLE-LIGHT ; ASSISTED SYNTHESIS ; TIO2 ; AG/TIO2 ; AG ; AG-TIO2 ; NANOCOMPOSITE ; NANOPARTICLES ; EFFICIENCY ; REDUCTION |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Key R&D Program of China[2018YFC1901200] ; National Natural Science Funds of China[51776211] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), China[GML2019ZD0101] |
WOS研究方向 | Engineering ; Materials Science ; Physics |
项目资助者 | National Key R&D Program of China ; National Natural Science Funds of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), China |
WOS类目 | Engineering, Electrical & Electronic ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
WOS记录号 | WOS:000535462600021 |
出版者 | ELSEVIER SCI LTD |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.giec.ac.cn/handle/344007/27119 |
专题 | 中国科学院广州能源研究所 |
通讯作者 | Yuan, Haoran |
作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China 3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 4.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 5.Foshan Univ, Coll Mat Sci & Energy Engn, Foshan 528000, Guangdong, Peoples R China 6.Chongqing Environm & Sanitat Grp Co Ltd, Chongqing 401121, Peoples R China |
第一作者单位 | 中国科学院广州能源研究所 |
推荐引用方式 GB/T 7714 | Shan, Rui,Lu, Lili,Gu, Jing,et al. Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions[J]. MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING,2020,114:12. |
APA | Shan, Rui.,Lu, Lili.,Gu, Jing.,Zhang, Yuyuan.,Yuan, Haoran.,...&Luo, Bo.(2020).Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions.MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING,114,12. |
MLA | Shan, Rui,et al."Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions".MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING 114(2020):12. |
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